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ZENG Fan, LI Yong, CHEN Shunqiang, ZHAO Xian, HU Hui, LIAO Li. Preparation of activated clay-stalk based activated carbon and its adsorption of COD in landfill leachate[J]. Chinese Journal of Environmental Engineering, 2017, 11(9): 5188-5194. doi: 10.12030/j.cjee.201609125
Citation: ZENG Fan, LI Yong, CHEN Shunqiang, ZHAO Xian, HU Hui, LIAO Li. Preparation of activated clay-stalk based activated carbon and its adsorption of COD in landfill leachate[J]. Chinese Journal of Environmental Engineering, 2017, 11(9): 5188-5194. doi: 10.12030/j.cjee.201609125
shu

Preparation of activated clay-stalk based activated carbon and its adsorption of COD in landfill leachate

  • 1.

    College of Environmental Science and Engineering, Huazhong University of Science and Technology, Wuhan 430074, China

  • 2.

    Department of Urban Construction Engineering, Wenhua College, Wuhan 430074, China

  • Received Date: 21/11/2016
    Accepted Date: 13/09/2016
    Available Online: 26/08/2017
    Fund Project:
  • Activated clay and corn stalk were used to prepare clay-stalk based activated carbon by high-temperature pyrolysis, and the activator was KOH. The physical and chemical properties and absorption characteristics of COD in landfill leachate were studied. The effects of activated carbon dosage, adsorption time and solution pH on COD removal were discussed and the adsorption isotherms were fitted. The results showed that an appropriate amount of activator could improve the iodine value and BET surface area of activated carbon, which could be 342.9 mg·g-1 and 420.34 m2·g-1 as the solid to alkali ratio was 0.4.The surface of the best carbon was irregular and porous, and porous structure was mainly mesoporous. The COD removal rate was 84%. The adsorption experimental data were fitted by both Langmuir and Freundlich isotherm models
  • [1] 周品,谷麟,饶姗姗,等.秸秆-污泥复合基活性炭的制备及其对1,2,4-酸氧体的吸附特性[J].环境化学,2013,32(1):106-111

    Google Scholar Pub Med

    [2] 史蕊,李依丽,尹晶,等. 玉米秸秆活性炭的制备及其吸附动力学研究[J]. 环境工程学报,2014,8(8):3428-3432

    Google Scholar Pub Med

    [3] 黄大成,王惠松,邹亚娟,等. 常压制备秸秆活性炭对水溶液中磷元素的吸附[J]. 环境工程学报,2015,9(3):1183-1188

    Google Scholar Pub Med

    [4] 何莹,舒威,廖筱锋,等.污泥-秸秆基活性炭的制备及其对渗滤液COD的吸附[J]. 环境工程学报,2015,9(4):1663-1669

    Google Scholar Pub Med

    [5] 陈友岚,李炳堂.污泥秸秆活性炭深度处理垃圾渗滤液的研究[J]. 环境污染与防治,2014,36(2):67-70

    Google Scholar Pub Med

    [6] RIVAS F J, BELTRAN F, CARVALHO F, et al. Study of different integrated physical-chemical+adsorption processes for landfill leachate remediation[J]. Industrial & Engineering Chemistry Research,2005,44(8):2871-2878

    Google Scholar Pub Med

    [7] RIVAS F J, BELTRAN F J, GIMENO O, et al. Adsorption of landfill leachates onto activated carbon:Equilibrium and kinetics[J]. Journal of Hazardous Materials,2006,131(1/2/3):170-178

    Google Scholar Pub Med

    [8] CHEN X, JEYASEELAN S, GRAHAM N. Physical and chemical properties study of the activated carbon made from sewage sludge[J]. Waste Management, 2002, 22(7):755-760

    Google Scholar Pub Med

    [9] OTERO M, ROZADA F, CALVO L F, et al. Elimination of organic water pollutants using adsorbents obtained from sewage sludge[J]. Dyes & Pigments, 2003, 57(1):55-65

    Google Scholar Pub Med

    [10] AHMADPOUR A, DO D D. The preparation of activated carbon from macadamia nutshell by chemical activation[J]. Carbon, 1997, 35(12):1723-1732

    Google Scholar Pub Med

    [11] KANG H Y, PARK S S, RIM Y S. Preparation of activated carbon from paper mill sludge by KOH-activation[J]. Korean Journal of Chemical Engineering, 2006, 23(6):948-953

    Google Scholar Pub Med

    [12] 谷麟, 周品, 袁海平, 等. 不同活化剂制备秸秆-污泥复配活性炭的机理及性能[J]. 净水技术, 2013, 32(2):61-66

    Google Scholar Pub Med

    [13] 谢招娣. 苎麻杆活性炭的制备及其应用研究[D]. 上海:东华大学, 2012

    Google Scholar Pub Med

    [14] 黄伟,贾艳秋,孙盛凯.活性炭及其改性研究进展[J].化学工业与工程技术,2006,27(5):39-44

    Google Scholar Pub Med

    [15] 何莹. 应用于H2S吸附的污泥-秸秆基活性炭的制备研究[D].武汉:华中科技大学,2015

    Google Scholar Pub Med

    [16] LENG C C, PINTO N G. Effects of surface properties of activated carbons on adsorption behavior of selected aromatics[J]. Carbon, 1997, 35(9):1375-1385

    Google Scholar Pub Med

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Preparation of activated clay-stalk based activated carbon and its adsorption of COD in landfill leachate

  • Received Date: 21/11/2016
  • Accepted Date: 13/09/2016
  • Available Online: 26/08/2017
Fund Project:

Abstract: Activated clay and corn stalk were used to prepare clay-stalk based activated carbon by high-temperature pyrolysis, and the activator was KOH. The physical and chemical properties and absorption characteristics of COD in landfill leachate were studied. The effects of activated carbon dosage, adsorption time and solution pH on COD removal were discussed and the adsorption isotherms were fitted. The results showed that an appropriate amount of activator could improve the iodine value and BET surface area of activated carbon, which could be 342.9 mg·g-1 and 420.34 m2·g-1 as the solid to alkali ratio was 0.4.The surface of the best carbon was irregular and porous, and porous structure was mainly mesoporous. The COD removal rate was 84%. The adsorption experimental data were fitted by both Langmuir and Freundlich isotherm models

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