Zhang Chengzhong, Ding Chao, Zhou Bianhong, Tao Li, Liu Lizhong. Pollution characteristics of carbon aerosol in PM2.5 of Xi’an during winter and summer[J]. Chinese Journal of Environmental Engineering, 2013, 7(4): 1477-1481.
Citation: Zhang Chengzhong, Ding Chao, Zhou Bianhong, Tao Li, Liu Lizhong. Pollution characteristics of carbon aerosol in PM2.5 of Xi’an during winter and summer[J]. Chinese Journal of Environmental Engineering, 2013, 7(4): 1477-1481.

Pollution characteristics of carbon aerosol in PM2.5 of Xi’an during winter and summer

  • Received Date: 02/03/2012
    Accepted Date: 19/12/2011
    Available Online: 09/04/2013
    Fund Project:
  • PM2.5 were collected by RP1400a instrument of TEOM series during winter and summer in Xi’an to study the variations of carbon aerosol, and the levels of organic carbon (OC), elemental carbon (EC) and water soluble carbon (WSOC) in samples were determined. The results showed that seasonal average concentrations of OC and EC in PM2.5 were higher in winter, the values were about 2.62 and 1.75 times of summer, respectively, which indicated that carbonaceous aerosol pollution was more serious in winter. The daily average concentrations of OC and EC presented double peak distribution in different seasons, that was mainly caused by the traffic source emissions and adverse weather conditions. The concentrations of OC and EC showed significant correlations in winter (R2 =0.823) and summer (R2=0.543), the average ratios of OC/EC were 5.36 and 3.58, respectively, which suggested that secondary organic carbon (SOC) were generated in the atmospheric particles.
  • [1] IPCC. Climate Change 1994: Radiative Forcing of Climate Change and An Evaluation of the IPCC IS92 Emission Scenarios. Cambridge University Press, New York, 1995

    Google Scholar Pub Med

    [2] Wilson R., Spengler J. D. Particle in Our Air: Eoncentrations and Health Effects. Harvard University Press, Cambridge, MA, 1996

    Google Scholar Pub Med

    [3] Wolff G.T. Particulate elemental carbon in the atmosphere. Journal of Air Pollution Control Association,1981,31(9):935-938

    Google Scholar Pub Med

    [4] Bizjak M., Tursic J., Lesnjak M., et al. Aerosol black carbon and ozone measurements at Mt. Krvavec EMEP/GAW station, Slovenia. Atmospheric Environment,1999,33(17):2783-2787

    Google Scholar Pub Med

    [5] Streets D. G., Gupta S., Waldho S. T., et al. Black carbon emissions in China. Atmospheric Environment,2001,35(25):4281-4296

    Google Scholar Pub Med

    [6] Yu Shaocai, Robin L. Dennis. Primary and secondary organic aerosols over the United States: Estimates on the basis of observed organic carbon (OC) and elemental carbon (EC), and air quality modeled primary OC/EC ratios. Atmospheric Environment,2004,38(31):5257-5268

    Google Scholar Pub Med

    [7] King A. M. New directions: TEOMs and the volatility of UK non-urban PM10: A regulatory dilemma.Atmospheric Environment,2000,34(19):3211-3212

    Google Scholar Pub Med

    [8] Vaida V., Tuck A. F., Ellison G. B. Optical and chemical properties of atmospheric organic aerosols. Physical Chemistry Earth, 2000,25(3):195-198

    Google Scholar Pub Med

    [9] Ravi Kant Pathak, Tao Wang, Ho K.F., et al. Characteristics of summertime PM2.5 organic and elemental carbon in four major Chinese cities: Implications of high acidity for water-soluble organic carbon (WSOC). Atmospheric Environment,2011,45(2):318-325

    Google Scholar Pub Med

    [10] Novakov T., Penner J. E. Large contribution of organic aerosols to cloud condensation nuclei concentrations. Nature, 1993,365(6449):823-826

    Google Scholar Pub Med

    [11] 许士玉,胡敏.气溶胶中的水溶性有机物研究进展. 环境科学研究,2000,13(1):50-53 Xu S.Y., Hu M. The advances of water-soluble or organic compounds in atmospheric particles. Research of Environmental Sciences, 2000,13(1):50-53(in Chinese)

    Google Scholar Pub Med

    [12] Saxena P., Hildemann L.M. Water-soluble organics in atmospheric particles:Acritical review of the literature and application of thermodynamics to identify Candidate compounds. Atmos. Chem., 1996,24(1):57-109

    Google Scholar Pub Med

    [13] Offenberg J. H., baker J. E. Aerosol size distribution of elemental and organic carbon in urban and over-water atmospheres. Atmospheric Environment, 2000,34(10):1509-1517

    Google Scholar Pub Med

    [14] 曹军骥,李顺诚,李杨,等.2003年秋冬季西安大气中有机碳和元素碳的理化特征及其来源解析. 自然科学进展,2005,15(12):1460-1466 Cao J.J., Lee S.C., Li Y., et al. The variability and source apportionment of organic carbon and elemental carbon in Xi’an atmosphere during the autumn and winter of 2003. Progress in Natural Science,2005,15(12):1460-1466(in Chinese)

    Google Scholar Pub Med

    [15] 吴琳,冯银厂,戴莉,等.天津市大气中 PM10、PM2.5 及其碳组分污染特征分析. 中国环境科学,2009,29(11):1134-1139 Wu L., Feng Y. C., Dai L. ,et al. Characteristics of PM10, PM2.5and their carbonaceous species in Tianjin City. China Environmental Science, 2009,29(11):1134-1139(in Chinese)

    Google Scholar Pub Med

    [16] Holler R., Tohnoa S., Kasraa M., et al. Long-term characterization of carbonaceous aerosol in Uji. Japan. Atmospheric Environment, 2002,36(8):1267-1275

    Google Scholar Pub Med

    [17] Seung Shik Park, Min S. Bae, James J. Schauer, et al. Evaluation of the TMO and TOT methods for OC and EC measurements and their characteristics in PM2.5 at an urban site of Korea during ACE-Asia. Atmospheric Environment,2005,39(28):5101-5112

    Google Scholar Pub Med

    [18] Can J. J., Lee S. C., Ho K. F., et al. Characteristics of carbonaceous aerosol in pearl river delta region, China during 2001 winter period. Atmosphere Environment,2003,37(11):1451-1460

    Google Scholar Pub Med

    [19] 于建华,虞统,杨晓光,等. 北京冬季PM2.5中元素碳、有机碳的污染特征. 环境科学研究,2004,17(1):48-51 Yu J. H., Yu T.,Yang X.G., et al. Characteristics of organic carbon and elemental carbon in PM2.5 in Beijing in the winter. Research of Environmental Sciences, 2004,17(1):48-51(in Chinese)

    Google Scholar Pub Med

    [20] Chow J.C., Waston J.G., Lu Z., et al. Descriptive analysis of PM2.5 and PM10 at regionally representative locations during SJVAQS/AUSPEX. Atmospheric Environment,1996,30(12):2079-2112

    Google Scholar Pub Med

    [21] 孟昭阳,张怀德,蒋晓明,等. 太原冬季PM2. 5中有机碳和元素碳的变化特征. 应用气象学报,2008,18(4):524-530 Meng Z. Y., Zhang H. D., Jiang X. M., et al. Characteristics of organic carbon and elemental carbon in PM2.5 during winter in Taiyuan. Journal of Applied Meteorological Science,2008,18(4):524-530(in Chinese)

    Google Scholar Pub Med

    [22] Rengarajan R., Sudheer A. K., Sarin M. M. Wintertime PM2.5 and PM10 carbonaceous and inorganic constituents from urban site in western India. Atmospheric Research,2011,102(4):420-431

    Google Scholar Pub Med

  • 加载中
通讯作者: 陈斌, bchen63@163.com
  • 1. 

    沈阳化工大学材料科学与工程学院 沈阳 110142

  1. 本站搜索
  2. 百度学术搜索
  3. 万方数据库搜索
  4. CNKI搜索

Article Metrics

Article views(1885) PDF downloads(1852) Cited by(0)

Access History

Pollution characteristics of carbon aerosol in PM2.5 of Xi’an during winter and summer

Fund Project:

Abstract: PM2.5 were collected by RP1400a instrument of TEOM series during winter and summer in Xi’an to study the variations of carbon aerosol, and the levels of organic carbon (OC), elemental carbon (EC) and water soluble carbon (WSOC) in samples were determined. The results showed that seasonal average concentrations of OC and EC in PM2.5 were higher in winter, the values were about 2.62 and 1.75 times of summer, respectively, which indicated that carbonaceous aerosol pollution was more serious in winter. The daily average concentrations of OC and EC presented double peak distribution in different seasons, that was mainly caused by the traffic source emissions and adverse weather conditions. The concentrations of OC and EC showed significant correlations in winter (R2 =0.823) and summer (R2=0.543), the average ratios of OC/EC were 5.36 and 3.58, respectively, which suggested that secondary organic carbon (SOC) were generated in the atmospheric particles.

Reference (22)

Catalog

/

DownLoad:  Full-Size Img  PowerPoint