亚硝酸盐对生物膜CANON工艺脱氮性能和N2O释放的影响

付昆明, 付巢, 王会芳, 苏雪莹, 李慧, 仇付国, 曹秀芹. 亚硝酸盐对生物膜CANON工艺脱氮性能和N2O释放的影响[J]. 环境工程学报, 2018, 12(10): 2776-2782. doi: 10.12030/j.cjee.201803181
引用本文: 付昆明, 付巢, 王会芳, 苏雪莹, 李慧, 仇付国, 曹秀芹. 亚硝酸盐对生物膜CANON工艺脱氮性能和N2O释放的影响[J]. 环境工程学报, 2018, 12(10): 2776-2782. doi: 10.12030/j.cjee.201803181
FU Kunming, FU Chao, WANG Huifang, SU Xueying, LI Hui, QIU Fuguo, CAO Xiuqin. Effects of nitrite on nitrogen removal performance and N2O emission in a biofilm CANON process[J]. Chinese Journal of Environmental Engineering, 2018, 12(10): 2776-2782. doi: 10.12030/j.cjee.201803181
Citation: FU Kunming, FU Chao, WANG Huifang, SU Xueying, LI Hui, QIU Fuguo, CAO Xiuqin. Effects of nitrite on nitrogen removal performance and N2O emission in a biofilm CANON process[J]. Chinese Journal of Environmental Engineering, 2018, 12(10): 2776-2782. doi: 10.12030/j.cjee.201803181

亚硝酸盐对生物膜CANON工艺脱氮性能和N2O释放的影响

  • 基金项目:

    北京市教育委员会科技发展计划项目(SQKM201710016006)

    北京建筑大学市属高校基本科研业务费专项资金(X18182,X18214)

Effects of nitrite on nitrogen removal performance and N2O emission in a biofilm CANON process

  • Fund Project:
  • 摘要: 通过调控进水NO2--N浓度分别为0、25、50和100 mg·L-1,研究不同初始NO2--N浓度对CANON工艺脱氮效果和N2O释放的影响。结果表明:SBBR中,初始NO2--N浓度分别为0、25、50和100 mg·L-1时,TN去除率分别达到81.65%、89.09%,87.75%和88.39%;对应的N2O释放率分别为7.03%、7.93%、10.21%和11.94%;前1/2周期内N2O释放量分别占总释放量的46%、53%、68%和75%。通过分析可知,较高初始NO2--N浓度,可以增加TN去除率,但是会刺激CANON工艺中N2O释放量的增加。
  • 加载中
  • [1] FUX C, BOEHLER M, HUBER P, et al.Biological treatment of ammonium-rich wastewater by partial nitritation and subsequent anaerobic ammonium oxidation (anammox) in a pilot plant[J].Journal of Biotechnology,2002,99(3):295-306 10.1016/S0168-1656(02)00220-1
    [2] LIANG Z, LIU J X.Landfill leachate treatment with a novel process: Anaerobic ammonium oxidation (anammox) combined with soil infiltration system[J].Journal of Hazardous Materials,2008,151(1):202-212 10.1016/j.jhazmat.2007.05.068
    [3] JOSS A, SALAGEBER D, EUGSTER J, et al.Full-scale nitrogen removal from digester liquid with partial nitritation and anammox in one SBR[J].Environmental Science & Technology,2009,43(14):5301-5306 10.1021/es900107w
    [4] OKABE S, OSHIKI M, TAKAHASHI Y, et al.N2O emission from a partial nitrification-anammox process and identification of a key biological process of N2O emission from anammox granules[J].Water Research,2011,45(19):6461-6470 10.1016/j.watres.2011.09.040
    [5] 王长科,罗新正,张华. 全球增温潜势和全球温变潜势对主要国家温室气体排放贡献估算的差异[J]. 气候变化研究进展,2013,9(1):49-54
    [6] PALUTIKOF B B Z K.Climate change and water.Technical paper of the intergovernmental panel on climate change, IPCC Secretariat[R].Geneva,2008
    [7] KIM S W, MIYAHARA M, FUSHINOBU S, et al.Nitrous oxide emission from nitrifying activated sludge dependent on denitrification by ammonia-oxidizing bacteria[J].Bioresource Technology,2010,101(11):3958-3963 10.1016/j.biortech.2010.01.030
    [8] POTH M, FOCHT D D. 15N kinetic analysis of N2O production by nitrosomonas europaea: An examination of nitrifier denitrification[J].Applied & Environmental Microbiology,1985,49(5):1134-1141
    [9] JIA W, LIANG S, ZHANG J, et al.Nitrous oxide emission in low-oxygen simultaneous nitrification and denitrification process: Sources and mechanisms[J].Bioresource Technology,2013,136(3):444-451 10.1016/j.biortech.2013.02.117
    [10] ZHOU Y, OEHMEN A, LIM M, et al.The role of nitrite and free nitrous acid (FNA) in wastewater treatment plants [J].Water Research,2011,45(15):4672-4682 10.1016/j.watres.2011.06.025
    [11] ALINSAFI A, ADOUANI N, BELINE F, et al.Nitrite effect on nitrous oxide emission from denitrifying activated sludge[J].Process Biochemistry,2008,43(6):683-689 10.1016/j.procbio.2008.02.008
    [12] 王会芳. 全程自养脱氮(CANON)工艺中N2O释放研究[D]. 北京:北京建筑大学,2016
    [13] 国家环境保护总局.水和废水监测分析方法[M]. 4版.北京:中国环境科学出版社,2002:63-64
    [14] ANTHONISEN A C, LOEH R C, PRAKASAM T B, et al.Inhibition of nitrification by ammonia and nitrous-acid[J].Journal Water Pollution Control Federation,1976,48(5):835-852 10.2307/25038971
    [15] 付昆明,王会芳,苏雪莹,等. 初始pH值对序批式CANON工艺脱氮效果和N2O释放的影响[J]. 环境科学,2016,37(11):4261-4267 10.13227/j.hjkx.201604221
    [16] 付昆明,张杰,曹相生,等.NH4+-N与NO2--N对连续流CANON反应器运行性能的影响[J]. 北京工业大学学报,2011,37(7):1038-1044
    [17] ZHANG D, CAI Q, CONG L.Enhancing completely autotrophic nitrogen removal over nitrite by trace NO2 addition to an AUSB reactor[J].Journal of Chemical Technology & Biotechnology,2010,85(2):204-208 10.1002/jctb.2288
    [18] ZU B, ZHANG D J, YAN Q.Effect of trace NO2 and kinetic characteristics for anaerobic ammonium oxidation of granular[J].Environmental Science,2008,29(3):683-687
    [19] 付昆明,张杰,曹相生,等. 改性聚乙烯填料CANON反应器的启动与运行[J]. 化工学报,2014,65(11):4406-4412
    [20] XIAO P Y, CAI Q, ZHANG D J, et al.Characteristics of nitrogen removal and nitrous oxide production in CANON process[J].Journal of Chemical Technology & Biotechnology,2014,89(4):552-558 10.1002/jctb.4153
    [21] SZATKOWSKA B, CEMA G, PLAZA E, et al.A one-stage system with partial nitritation and anammox processes in the moving-bed biofilm reactor[J].Water Science & Technology,2007,55(8/9):19-26 10.2166/wst.2007.237
    [22] POTH M.Dinitrogen production from nitrite by a nitrosomonas isolate[J].Applied & Environmental Microbiology,1986,52(4):957-959
    [23] ZHOU Y, PIJUAN M, ZENG R J, et al.Free nitrous acid inhibition on nitrous oxide reduction by a denitrifying-enhanced biological phosphorus removal sludge[J].Environmental Science & Technology,2008,42(22):8260-8265 10.1021/es800650j
    [24] YUE J, WANG D, ZHANG W.Effects of substrates on N2O emissions in an anaerobic ammonium oxidation (anammox) reactor[J].Springerplus,2016,5(1):741-752 10.1186/s40064-016-2392-1
  • 加载中
计量
  • 文章访问数:  2501
  • HTML全文浏览数:  2337
  • PDF下载数:  160
  • 施引文献:  0
出版历程
  • 刊出日期:  2018-10-11

亚硝酸盐对生物膜CANON工艺脱氮性能和N2O释放的影响

  • 1. 北京建筑大学环境与能源工程学院,城市雨水系统与水环境教育部重点实验室,中-荷污水处理技术研发中心,北京 100044
  • 2. 北京城市排水集团有限责任公司科技研发中心,北京 100032
基金项目:

北京市教育委员会科技发展计划项目(SQKM201710016006)

北京建筑大学市属高校基本科研业务费专项资金(X18182,X18214)

摘要: 通过调控进水NO2--N浓度分别为0、25、50和100 mg·L-1,研究不同初始NO2--N浓度对CANON工艺脱氮效果和N2O释放的影响。结果表明:SBBR中,初始NO2--N浓度分别为0、25、50和100 mg·L-1时,TN去除率分别达到81.65%、89.09%,87.75%和88.39%;对应的N2O释放率分别为7.03%、7.93%、10.21%和11.94%;前1/2周期内N2O释放量分别占总释放量的46%、53%、68%和75%。通过分析可知,较高初始NO2--N浓度,可以增加TN去除率,但是会刺激CANON工艺中N2O释放量的增加。

English Abstract

参考文献 (24)

目录

/

返回文章
返回