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纳秒脉冲电源下电晕放电去除苯乙烯

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刘百良, 李驰波, 黄逸凡, 闫克平, 刘振. 纳秒脉冲电源下电晕放电去除苯乙烯[J]. 环境工程学报, 2018, 12(1): 145-152. doi: 10.12030/j.cjee.201706009
引用本文: 刘百良, 李驰波, 黄逸凡, 闫克平, 刘振. 纳秒脉冲电源下电晕放电去除苯乙烯[J]. 环境工程学报, 2018, 12(1): 145-152. doi: 10.12030/j.cjee.201706009
shu
LIU Bailiang, LI Chibo, HUANG Yifan, YAN Keping, LIU Zhen. Styrene removal using corona discharge combined with nanosecond pulse power supply[J]. Chinese Journal of Environmental Engineering, 2018, 12(1): 145-152. doi: 10.12030/j.cjee.201706009
Citation: LIU Bailiang, LI Chibo, HUANG Yifan, YAN Keping, LIU Zhen. Styrene removal using corona discharge combined with nanosecond pulse power supply[J]. Chinese Journal of Environmental Engineering, 2018, 12(1): 145-152. doi: 10.12030/j.cjee.201706009
shu

纳秒脉冲电源下电晕放电去除苯乙烯

  • 1.

    浙江大学化学工程与生物工程学院,工业生态与环境研究所,杭州 310028

  • 基金项目:

    国家自然科学基金资助项目 (21276232)

Styrene removal using corona discharge combined with nanosecond pulse power supply

  • 1.

    Industrial Ecological and Environmental Research Institute, College of Chemical and Biological Engineering, Zhejiang University, Hangzhou 310028,China

  • Fund Project:

  • 摘要: 设计一套纳秒量级的脉冲电源,测试结果表明脉冲上升沿为15 ns,脉宽30 ns,输出端串联后最大峰值电压为20 kV,并联后最大峰值电流为340 A。电源频率在50~600 Hz范围内变化且输出脉冲的极性可调节。纳秒脉冲源匹配反应器后产生电晕放电,在相同的电源输出能量下,负脉冲的能量注入效率只有37.4%,而正脉冲为87.3%。当脉冲频率为600 Hz时,反应器功率为59.4 W。以苯乙烯为目标处理物,当能量密度为27.4 J·L-1 时,苯乙烯降解效率达到98.6%。相同能量密度下,负脉冲放电下苯乙烯的去除率最高。
    Abstract: An efficient and reliable pulsed power generator is developed both in circuit principle and design implementation. Experimental results show that the rising edge of the pulse is 15 ns, pulse width is 30 ns. The maximum peak voltage is 20 kV when the output is connected in series, the maximum peak current after parallel is 340 A. The power supply frequency varies from 50 to 600 Hz and the polarity of the output pulse can be adjusted. At the same output energy, the efficiency of negative pulse is only 37.4%, while positive pulse is 87.3%. When the pulse frequency is 600 Hz, the reactor power is 59.4 W. When the energy density is 27.4 J·L-1, the degradation efficiency of styrene reaches 98.6%. At the same energy density, the removal rate of styrene under negative pulse discharge is higher than positive pulse.
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  • [1] GONG Y, WEI Y, CHENG J, et al.Health risk assessment and personal exposure to volatile organic compounds (VOCs) in metro carriages:A case study in Shanghai, China[J].Science of the Total Environment,2016,4:1432-1438
    [2] 闫克平, 李树然, 冯卫强,等.高电压环境工程应用研究关键技术问题分析及展望[J].高电压技术,2015,1(8):2528-2544
    [3] KARATUM O, DESHUSSES M A.A comparative study of dilute VOCs treatment in a non-thermal plasma reactor[J].Chemical Engineering Journal,2016,4:308-315
    [4] 聂勇, 汪晶毅, 钟侃,等.等离子体辅助催化还原NOx系统的优化[J].高电压技术,2008,4(2):359-362
    [5] CLODFELTER W H, BASU S, BOLDEN C, et al.The relationship between plasma and salivary NOx[J].Nitric Oxide,2015,7:85-90
    [6] FALCH A, LATES V, KRIEK R J.Combinatorial plasma sputtering of PtePdy, thin film electrocatalysts for aqueous SO2,electro-oxidation[J].Electrocatalysis,2015,6(3):1-9
    [7] BAI M, LENG B, MAO S, et al.Flue gas desulfurization by dielectric barrier discharge[J].Plasma Chemistry and Plasma Processing,2016,6(2):511-521
    [8] CHOUEIRI E Y, POLZIN K A.Faraday acceleration with radio-frequency assisted discharge[J].Journal of Propulsion & Power,2015,2(3):611-619
    [9] LI B, CHEN Q, LIU Z W.A large gap of radio frequency dielectric barrier atmospheric pressure glow discharge[J].Applied Physics Letters,2010,6(4):453-460
    [10] LI X, YUAN N, NIU D, et al.Current measurements and diagnosis on dielectric barrier discharge in a coaxial geometry at atmospheric pressure[C]//IEEE Computer Society.International Conference on Electrical and Control Engineering, 2010:652-655
    [11] YAMAMOTO T, OKUBO M.Nonthermal Plasma Technology[M].Totowa, NJ:The Humana Press Inc.,2007:135-293
    [12] DURME J V, DEWULF J, SYSMANS W, et al.Abatement and degradation pathways of toluene in indoor air by positive corona discharge[J].Chemosphere,2007,8(10):1821-1829
    [13] LIU Z Q, WANG J G, QING L I, et al.Study on spray characteristics of corona discharge on cavity-type hydro pole[J].Transactions of Beijing Institute of Technology,2011,1(1):78-82
    [14] TOCHIKUBO F, FURUTA Y, UCHIDA S, et al.Study of wastewater treatment by OH radicals using DC and pulsed corona discharge over water[J].Japanese Journal of Applied Physics,2006,5(4A):2743-2748
    [15] XU X, GAO X, YAN P, et al.Particle migration and collection in a high-temperature electrostatic precipitator[J].Separation & Purification Technology,2015,3:184-191
    [16] HENSEL K, KUACˇGEROV K, TARABOV B, et al.Effects of air transient spark discharge and helium plasma jet on water, bacteria, cells, and biomolecules[J].Biointerphases,2015,0(2):029515.DOI:10.1116/1.4919559
    [17] 王翔, 常景彩.线-板式静电除尘器芒刺电晕线放电特性[J].高电压技术,2017,3(2):533-540
    [18] GOLUBOVSKII Y B, MAIOROV V A, BEHNKE J F, et al.Study of the homogeneous glow-like discharge in nitrogen at atmospheric pressure[J].Journal of Physics D:Applied Physics,2004,7(9):1346-1356
    [19] ZHANG X, ZHU J, LI X, et al.Characteristics of styrene removal with estreamer corona plasma system[J].IEEE Transactions on Plasma Science,2011,9(6):1482-1488
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  • 刊出日期:  2018-01-14
刘百良, 李驰波, 黄逸凡, 闫克平, 刘振. 纳秒脉冲电源下电晕放电去除苯乙烯[J]. 环境工程学报, 2018, 12(1): 145-152. doi: 10.12030/j.cjee.201706009
引用本文: 刘百良, 李驰波, 黄逸凡, 闫克平, 刘振. 纳秒脉冲电源下电晕放电去除苯乙烯[J]. 环境工程学报, 2018, 12(1): 145-152. doi: 10.12030/j.cjee.201706009
shu
LIU Bailiang, LI Chibo, HUANG Yifan, YAN Keping, LIU Zhen. Styrene removal using corona discharge combined with nanosecond pulse power supply[J]. Chinese Journal of Environmental Engineering, 2018, 12(1): 145-152. doi: 10.12030/j.cjee.201706009
Citation: LIU Bailiang, LI Chibo, HUANG Yifan, YAN Keping, LIU Zhen. Styrene removal using corona discharge combined with nanosecond pulse power supply[J]. Chinese Journal of Environmental Engineering, 2018, 12(1): 145-152. doi: 10.12030/j.cjee.201706009
shu

纳秒脉冲电源下电晕放电去除苯乙烯

  • 1. 浙江大学化学工程与生物工程学院,工业生态与环境研究所,杭州 310028
基金项目:

国家自然科学基金资助项目 (21276232)

摘要: 设计一套纳秒量级的脉冲电源,测试结果表明脉冲上升沿为15 ns,脉宽30 ns,输出端串联后最大峰值电压为20 kV,并联后最大峰值电流为340 A。电源频率在50~600 Hz范围内变化且输出脉冲的极性可调节。纳秒脉冲源匹配反应器后产生电晕放电,在相同的电源输出能量下,负脉冲的能量注入效率只有37.4%,而正脉冲为87.3%。当脉冲频率为600 Hz时,反应器功率为59.4 W。以苯乙烯为目标处理物,当能量密度为27.4 J·L-1 时,苯乙烯降解效率达到98.6%。相同能量密度下,负脉冲放电下苯乙烯的去除率最高。

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