给水污泥对水中磷的吸附性能

徐颖, 叶志隆, 叶欣, 吴杰, 林向宇. 给水污泥对水中磷的吸附性能[J]. 环境工程学报, 2018, 12(3): 712-719. doi: 10.12030/j.cjee.201708032
引用本文: 徐颖, 叶志隆, 叶欣, 吴杰, 林向宇. 给水污泥对水中磷的吸附性能[J]. 环境工程学报, 2018, 12(3): 712-719. doi: 10.12030/j.cjee.201708032
XU Ying, YE Zhilong, YE Xin, WU Jie, LIN Xiangyu. Phosphorus adsorption performance of water-supply sludge[J]. Chinese Journal of Environmental Engineering, 2018, 12(3): 712-719. doi: 10.12030/j.cjee.201708032
Citation: XU Ying, YE Zhilong, YE Xin, WU Jie, LIN Xiangyu. Phosphorus adsorption performance of water-supply sludge[J]. Chinese Journal of Environmental Engineering, 2018, 12(3): 712-719. doi: 10.12030/j.cjee.201708032

给水污泥对水中磷的吸附性能

  • 基金项目:

    厦门市科技计划项目(3502Z20162002)

    福建省科技计划项目(2013YZ0001-1)

Phosphorus adsorption performance of water-supply sludge

  • Fund Project:
  • 摘要: 以给水污泥为磷的吸附材料,采用静态吸附和动态吸附方法对比研究了干、湿状态下给水污泥对磷的吸附特性。静态吸附实验结果表明,给水污泥对磷的吸附过程以化学吸附为主,满足Freundlich等温吸附方程式。在300?K条件下,原始状态的湿污泥相比烘干后的污泥能更快地达到磷吸附平衡,且具有更高的理论饱和吸附量,分别为3.487?mg·g-1(相当于11.710?mg·g-1,以干污泥计)和9.832?mg·g-1。长期动态吸附实验结果表明,原始状态的给水污泥对磷的实际饱和吸附量为3.065?mg·g-1,接近理论饱和吸附量。因此,原始状态的给水污泥可直接用作除磷材料,无需预先烘干处理。
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  • [1] SCHINDLER D W, HECKY R, FINDLAY D, et al.Eutrophication of lakes cannot be controlled by reducing nitrogen input: results of a 37-year whole-ecosystem experiment[J].Proceedings of the National Academy of Sciences, 2008,105(32):11254-11258
    [2] 刘霄, 黄岁樑, 刘学功. 3种人工湿地基质对磷的吸附特性[J]. 环境工程学报, 2012,6(10):3367-3372
    [3] 曾德芳, 徐保林. 沉淀-絮凝结合法处理磷化废水的研究[J]. 环境工程学报, 2009,3(5):795-798
    [4] OEHMEN A, LEMOS P C, CARVALHO G, et al.Advances in enhanced biological phosphorus removal: From micro to macro scale[J].Water Research,2007,41(11):2271-2300 10.1016/j.watres.2007.02.030
    [5] 唐朝春, 刘名, 陈惠民, 等. 吸附除磷技术的研究进展[J]. 水处理技术,2014,40(9):1-7
    [6] YANG S, DING D, ZHAO Y, et al.Investigation of phosphate adsorption from aqueous solution using Kanuma mud: Behaviors and mechanisms[J].Journal of Environmental Chemical Engineering,2013,1(3):355-362 10.1016/j.jece.2013.05.016
    [7] YOON S Y, LEE C G, PARK J A, et al.Kinetic, equilibrium and thermodynamic studies for phosphate adsorption to magnetic iron oxide nanoparticles[J].Chemical Engineering Journal,2014,236(2):341-347 10.1016/j.cej.2013.09.053
    [8] NAMASIVAYAM C, PRATHAP K.Recycling Fe(III)/Cr(III) hydroxide, an industrial solid waste for the removal of phosphate from water[J].Journal of Hazardous Materials,2005,123(1/2/3):127-134 10.1016/j.jhazmat.2005.03.037
    [9] KUMAR P, SUDHA S, CHAND S, et al.Phosphate removal from aqueous solution using coir-pith activated carbon[J].Separation Science & Technology,2010,45(10):1463-1470 10.1080/01496395.2010.485604
    [10] 王勤华, 贺俊兰. 净水厂产泥量的确定和相关参数的选择[J]. 中国给水排水,2002,18(8):64-66 10.3321/j.issn:1000-4602.2002.08.022
    [11] 袁东海, 景丽洁, 张孟群, 等. 几种人工湿地基质净化磷素的机理[J]. 中国环境科学,2004,24(5):614-617 10.3321/j.issn:1000-6923.2004.05.025
    [12] YANG Y, TOMLINSON D, KENNEDY S, et al.Dewatered alum sludge: A potential adsorbent for phosphorus removal[J].Water Science & Technology,2006,54(5):207-213 10.2166/wst.2006.564
    [13] 马啸宙, 魏东洋, 马宏林, 等. 基于给水污泥吸附水溶液中磷的影响因素[J]. 环境工程学报,2015,9(8):3659-3666
    [14] 王信, 马啸宙, 周雯, 等. 给水污泥负载Fe合物除磷行为效果及机理[J]. 环境工程学报, 2016,10(10):5420-5428 10.12030/j.cjee.201602116
    [15] 高思佳, 王昌辉, 裴元生. 热活化和酸活化给水处理厂废弃铁铝泥的吸磷效果[J]. 环境科学学报,2012,32(3):606-611
    [16] 国家环境保护总局.水和废水监测分析方法[M]. 4版.北京:中国环境科学出版社, 2002
    [17] DRIZO A, FROST C A, GRACE J, et al.Physico-chemical screening of phosphate-removing substrates for use in constructed wetland systems[J].Water Research,1999,33(17):3595-3602 10.1016/S0043-1354(99)00082-2
    [18] BUBBA M D, ARIAS C A, BRIX H.Phosphorus adsorption maximum of sands for use as media in subsurface flow constructed reed beds as measured by the Langmuir isotherm[J].Water Research,2003,37(14):3390-3400 10.1016/S0043-1354(03)00231-8
    [19] STRANG T J, WAREHAM D G.Phosphorus removal in a waste-stabilization pond containing limestone rock filters[J].Journal of Environmental Engineering & Science,2006,5(6):447-457 10.1139/s06-017
    [20] YANG Y, ZHAO Y Q, BABATUNDE A O, et al.Characteristics and mechanisms of phosphate adsorption on dewatered alum sludge[J].Separation & Purification Technology,2006,51(2):193-200 10.1016/j.seppur.2006.01.013
    [21] BABATUNDE A O, ZHAO Y Q, BURKE A M, et al.Characterization of aluminium-based water treatment residual for potential phosphorus removal in engineered wetlands[J].Environmental Pollution,2009,157(10):2830-2836 10.1016/j.envpol.2009.04.016
    [22] 程爱华, 尹向辉, 杨磊. 给水厂污泥吸附磷的动力学和热力学研究[J]. 绿色科技,2013(2):129-131 10.3969/j.issn.1674-9944.2013.02.053
    [23] 操家顺, 朱文杰, 李超, 等. 给水厂污泥作为人工湿地滤料对磷的去除效果研究[J]. 环境科技,2015,28(5):16-20 10.3969/j.issn.1674-4829.2015.05.006
    [24] BABATUNDE A O, ZHAO Y Q.Equilibrium and kinetic analysis of phosphorus adsorption from aqueous solution using waste alum sludge[J].Journal of Hazardous Materials,2010,184(1/2/3):746-752 10.1016/j.jhazmat.2010.08.102
    [25] SAKADEVAN K, BAVOR H J.Phosphate adsorption characteristics of soils, slags and zeolite to be used as substrates in constructed wetland systems[J].Water Research, 1998,32(2):393-399 10.1016/S0043-1354(97)00271-6
    [26] SUKSABYE P, THIRAVETYAN P, NAKBANPOTE W.Column study of chromium(VI) adsorption from electroplating industry by coconut coir pith[J].Journal of Hazardous Materials,2008,160(1):56-62 10.1016/j.jhazmat.2008.02.083
    [27] 王振. 潜流人工湿地对养猪废水处理效能的强化及其稳定性研究[D].北京:中国科学院大学,2013
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出版历程
  • 刊出日期:  2018-03-22

给水污泥对水中磷的吸附性能

  • 1. 中国科学院城市污染物转化重点实验室,厦门361021
  • 2. 中国科学院城市环境研究所,厦门361021
基金项目:

厦门市科技计划项目(3502Z20162002)

福建省科技计划项目(2013YZ0001-1)

摘要: 以给水污泥为磷的吸附材料,采用静态吸附和动态吸附方法对比研究了干、湿状态下给水污泥对磷的吸附特性。静态吸附实验结果表明,给水污泥对磷的吸附过程以化学吸附为主,满足Freundlich等温吸附方程式。在300?K条件下,原始状态的湿污泥相比烘干后的污泥能更快地达到磷吸附平衡,且具有更高的理论饱和吸附量,分别为3.487?mg·g-1(相当于11.710?mg·g-1,以干污泥计)和9.832?mg·g-1。长期动态吸附实验结果表明,原始状态的给水污泥对磷的实际饱和吸附量为3.065?mg·g-1,接近理论饱和吸附量。因此,原始状态的给水污泥可直接用作除磷材料,无需预先烘干处理。

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