某废弃铀矿周边农田土壤重金属和放射性元素的风险分析和修复措施

施宸皓, 梁婕, 曾光明, 袁玉洁, 钟敏洲, 张立华. 某废弃铀矿周边农田土壤重金属和放射性元素的风险分析和修复措施[J]. 环境工程学报, 2018, 12(1): 213-219. doi: 10.12030/j.cjee.201701006
引用本文: 施宸皓, 梁婕, 曾光明, 袁玉洁, 钟敏洲, 张立华. 某废弃铀矿周边农田土壤重金属和放射性元素的风险分析和修复措施[J]. 环境工程学报, 2018, 12(1): 213-219. doi: 10.12030/j.cjee.201701006
SHI Chenhao, LIANG Jie, ZENG Guangming, YUAN Yujie, ZHONG Minzhou, ZHANG Lihua. Assessment of heavy metal and radionuclide pollution risk in farmland around an abandoned uranium mine and its related remediation measures[J]. Chinese Journal of Environmental Engineering, 2018, 12(1): 213-219. doi: 10.12030/j.cjee.201701006
Citation: SHI Chenhao, LIANG Jie, ZENG Guangming, YUAN Yujie, ZHONG Minzhou, ZHANG Lihua. Assessment of heavy metal and radionuclide pollution risk in farmland around an abandoned uranium mine and its related remediation measures[J]. Chinese Journal of Environmental Engineering, 2018, 12(1): 213-219. doi: 10.12030/j.cjee.201701006

某废弃铀矿周边农田土壤重金属和放射性元素的风险分析和修复措施

  • 基金项目:

    〖ZK

Assessment of heavy metal and radionuclide pollution risk in farmland around an abandoned uranium mine and its related remediation measures

  • Fund Project:
  • 摘要: 在某废弃的铀矿周围农田选取10个土壤样点,采集表层土壤下(0~60 cm)不同深度的60个土壤样品,分析其中重金属和放射性元素污染水平,并进行污染修复方案设计。结果表明:Pb、Cd、Cu、Zn、As、Hg、Cr、Mn、Ni、U和232Th的平均浓度分别为2 275.69、6.09、71.51、1 230.47、47.87、502.81、46.22、422.39、12.01、74.05和27.28 mg·kg-1,Pb、Cd、Cu、Zn、As、Hg和U的浓度高于研究区域土壤环境背景值,原采矿场和原堆积矿场是重点污染区域;地累积指数(Igeo)显示农田Hg处于高污染水平,Cd、Zn、Pb和U处于中度污染水平以上。采用覆土、钝化和植物修复相结合的方法进行原矿区场地修复。在原矿区场地加入钝化剂或植物提取修复之前进行覆土。结果表明原采矿场、原堆积矿场分别覆土140和120 cm,氡析出率≤0.74 Bq·(m2·s)-1,γ射线剂量率接近30×10-8 Gy·h-1。结果满足环境标准要求。
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  • [1] MAO L J, MO D W, FU Q, et al.Multivariate analysis of heavy metals in surface sediments from lower reaches of the Xiangjiang River, southern China[J].Environmental Earth Sciences,2013,9(3):765-771
    [2] ZHOU J, MA D S, PAN J Y, et al.Application of multivariate statistical approach to identify heavy metal sources in sediment and waters:A case study in Yangzhong, China[J].Environmental Geology,2008,4(2):373-380
    [3] ZHU H N, YUAN X Z, ZENG G M, et al.Ecological risk assessment of heavy metals in sediments of Xiawan Port based on modified potential ecological risk index[J].Transactions of Nonferrous Metals Society China,2012,2(6):1470-1477
    [4] ZHANG C, NIE S, LIANG J, et al.Effects of heavy metals and soil physicochemical properties on wetland soil microbial biomass and bacterial community structure[J].Science of the Total Environment,2016,7-558:785-790
    [5] HUANG D L, ZENG G M, FENG C L, et al.Degradation of lead-contaminated lignocellulosic waste by Phanerochaete chrysosporium and the reduction of lead toxicity[J].Environmental Science & Technology,2008,2(13):4946-4951
    [6] TANG L, ZENG G M, SHEN G L, et al.Rapid detection of picloram in agricultural field samples using a disposable immunomembrane-based electrochemical sensor[J].Environmental Science and Technology,2008,2(4):1207-1212
    [7] RENZONI A, ZINO F, FRANCHI E.Mercury levels along the food chain and risk for exposed populations[J].Environmental Research,1998,7(2):68-72
    [8] DUDKA S, MILLER W P.Accumulation of potentially toxic elements in plants and their transfer to human food chain[J].Journal of Environmental Science and Health:Part B,1999,4(4):681-708
    [9] PERALTA-VIDEA J R, LOPEZ M L, NARAYAN M, et al.The biochemistry of environmental heavy metal uptake by plants:Implications for the food chain[J].Internal Journal of Biochemistry & Cell Biology,2009,1(8/9):1665-1677
    [10] LIU J Y, LIANG J, YUAN X Z, et al.An integrated model for assessing heavy metal exposure risk to migratory birds in wetland ecosystem:A case study in Dongting Lake Wetland, China[J].Chemosphere,2015,5:14-19
    [11] LIANG J, LIU J Y, YUAN X Z, et al.A method for heavy metal exposure risk assessment to migratory herbivorous birds and identification of priority pollutants/areas in wetlands[J].Environmental Science and Pollution Research,2016,3(12):11806-11813
    [12] AL-TRABULSY H A, KHATER A E M, HABBANI F I.Radioactivity levels and radiological hazard indices at the Saudi coastline of the Gulf of Aqaba[J].Radiation Physics and Chemistry,2011,0(9):343-348
    [13] KANNANA V, RAJANA M P, IYENGARA M A R, et al.Distribution of natural and antropogenia radionuclides in soil and beach sand simples of Kalpakkam (India) using hyper pure germanium (HPGe) gamma ray spectrometry[J].Applied Radiation and Isotopes,2002,7(1):109-119
    [14] ZHANG X Y, LIN F F, WONG M T F, et al.Identification of soil heavy metal sources from anthropogenic activities and pollution assessment of Fuyang County, China[J].Environmental Monitoring and Assessment,2009,4:439-449
    [15] DOSSETO A, BUSS H L, SURESH P O.Rapid regolith formation over volcanic bedrock and implications for landscape evolution[J].Earth & Planetary Science Letters,2012,7(4):47-55
    [16] KEECH A R, WEST A J, PETT-RIDGE J C, et al.Evaluating U-series tools for weathering rate and duration on a soil sequence of known ages[J].Earth & Planetary Science Letters,2013,4(4):24-35
    [17] CHABAUX F, BLAES E, ROUPERT R, et al.Regolith formation rate from U-series nuclides:Implications from the study of a spheroidal weathering profile in the Rio Icacos watershed (Puerto Rico) [J].Geochimica et Cosmochimica Acta,2013,0(5):73-95
    [18] TASKIN H, KARAVUS M, AY P, et al.Radionuclide concentrations in soil and lifetime cancer risk due to gamma radioactivity in Kirklareli, Turkey[J].Journal of Environmental Radioactivity,2009,0(1):49-53
    [19] BLEISE A, DANESI P R, BURKART W.Properties, use and health effects of depleted uranium (DU):A general overview[J].Journal of Environmental Radioactivity,2003,4(2/3):93-112
    [20] ABBASPOUR M, MOATTAR F, OKHOVATIAN A, et al.Relationship of soil terrestrial radionuclide concentrations and the excess of lifetime cancer risk in western Mazandaran province, Iran[J].Radiation Protection Dosimetry,2010,2(2/3/4):265-272
    [21] WEISS H A, DARBY S C, DOLL R.Cancer mortality following X-ray treatment for ankylosing spondylitis[J].International Journal of Cancer,1994,9(3):327-338
    [22] CHEN C W, KAO C M, CHEN C F, et al.Distribution and accumulation of heavy metals in the sediments of Kaohsiung Harbor, Taiwan[J].Chemosphere,2007,6(8):1431-1440
    [23] BAI H, HU B T, WANG C G, et al.Assessment of radioactive materials and heavy metals in the surface soil around uranium mining area of Tongliao, China[J].Ecotoxicolgy and Environmental Safety,2016,0(8):185-192
    [24] PRAVEENA S M, AHMED A, RADOJEVIC M, et al.Heavy metals in mangrove surface sediment of Mengkabong Lagoon, Sabah:Multivariate and geo-accumulation index approaches[J].Bulletin of Environmental Contamination and Toxicology,2008,1(1):52-56
    [25] LIU P H, WEI C S, ZHANG S M, et al.Assessment on radioactive uranium contamination of paddy soil in uranium mine at southeast China by ICP-MS[J].Asian Journal of Chemistry,2015,7(3):1049-1052
    [26] JELLISS P A, BUCKNER S W, CHUNG S W, et al.The use of 1,2-epoxyhexane as a passivating agent for core-shell aluminum nanoparticles with very high active aluminum content[J].Solid State Sciences,2013,3(3):8-12
    [27] 黎大荣, 吴丽香, 宁晓君, 等.不同钝化剂对土壤有效态铅和镉含量的影响[J].环境保护科学,2013,9(3):46-49
    [28] 施培俊, 王冠华, 吴迪, 等.几种有机、无机钝化剂对铜污染土壤的钝化效果研究[J].环境工程,2016,4(6):173-176
    [29] 殷飞, 王海娟, 李燕燕, 等.不同钝化剂对重金属复合污染土壤的修复效应研究[J].农业环境科学学报,2015,4(3):438-448
    [30] 姜华, 吴波, 李国学.添加不同钝化剂降低污泥堆肥的植物毒性研究[J].环境工程学报,2008,2(10):1413-1415
    [31] CAMERON K C, DI H J, MOIR J L, et al.Nitrogen losses from the soil/plant system:A review[J].Solid State Sciences,2013,2(2):145-173
    [32] WANG H, STUANES A Q.Heavy metal pollution in air-water-soil-plant system of Zhuzhou City, Hunan Province, China[J].Water, Air, & Soil Pollution,2003,7(1):79-107
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  • 刊出日期:  2018-01-14

某废弃铀矿周边农田土壤重金属和放射性元素的风险分析和修复措施

  • 1. 核工业北京地质研究院,北京 100029
  • 2. 湖南大学环境科学与工程学院,长沙 410082
基金项目:

〖ZK

摘要: 在某废弃的铀矿周围农田选取10个土壤样点,采集表层土壤下(0~60 cm)不同深度的60个土壤样品,分析其中重金属和放射性元素污染水平,并进行污染修复方案设计。结果表明:Pb、Cd、Cu、Zn、As、Hg、Cr、Mn、Ni、U和232Th的平均浓度分别为2 275.69、6.09、71.51、1 230.47、47.87、502.81、46.22、422.39、12.01、74.05和27.28 mg·kg-1,Pb、Cd、Cu、Zn、As、Hg和U的浓度高于研究区域土壤环境背景值,原采矿场和原堆积矿场是重点污染区域;地累积指数(Igeo)显示农田Hg处于高污染水平,Cd、Zn、Pb和U处于中度污染水平以上。采用覆土、钝化和植物修复相结合的方法进行原矿区场地修复。在原矿区场地加入钝化剂或植物提取修复之前进行覆土。结果表明原采矿场、原堆积矿场分别覆土140和120 cm,氡析出率≤0.74 Bq·(m2·s)-1,γ射线剂量率接近30×10-8 Gy·h-1。结果满足环境标准要求。

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