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磁性OMS-2/SBR耦合处理活性染料X-3B废水

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喻阳, 钟笑涵, 徐爱华, 夏东升, 曾庆福, 潘飞. 磁性OMS-2/SBR耦合处理活性染料X-3B废水[J]. 环境工程学报, 2016, 10(10): 5555-5560. doi: 10.12030/j.cjee.201504029
引用本文: 喻阳, 钟笑涵, 徐爱华, 夏东升, 曾庆福, 潘飞. 磁性OMS-2/SBR耦合处理活性染料X-3B废水[J]. 环境工程学报, 2016, 10(10): 5555-5560. doi: 10.12030/j.cjee.201504029
shu
YU Yang, ZHONG Xiaohan, XU Aihua, XIA Dongsheng, ZENG Qingfu, PAN Fei. Advanced treatment of simulated X-3B wastewater by coupling magnetic OMS-2 with SBR[J]. Chinese Journal of Environmental Engineering, 2016, 10(10): 5555-5560. doi: 10.12030/j.cjee.201504029
Citation: YU Yang, ZHONG Xiaohan, XU Aihua, XIA Dongsheng, ZENG Qingfu, PAN Fei. Advanced treatment of simulated X-3B wastewater by coupling magnetic OMS-2 with SBR[J]. Chinese Journal of Environmental Engineering, 2016, 10(10): 5555-5560. doi: 10.12030/j.cjee.201504029
shu

磁性OMS-2/SBR耦合处理活性染料X-3B废水

  • 1.

    武汉纺织大学环境工程学院, 武汉 430073

  • 2.

    武汉纺织大学生态苎麻产业关键技术湖北省协同创新中心, 武汉 430073

  • 基金项目:

    国家科技支撑计划课题（2014BAC13B02）

    湖北省教育厅中青年项目（Q20151603）

  • 中图分类号: X703

Advanced treatment of simulated X-3B wastewater by coupling magnetic OMS-2 with SBR

  • 1.

    School of Environmental Engineering, Wuhan Textile University, Wuhan 430073, China

  • 2.

    Collaborative Innovation Center for Key Technology of Ecological Ramie Industrialization, Hubei Province, Wuhan Textile University, Wuhan 430073, China

  • Fund Project:

摘要

  • 摘要: 为了深度处理印染废水，将基于硫酸根自由基的高级氧化法与序批式活性污泥法（SBR）相耦合；采用磁性氧化锰八面体分子筛（OMS-2）作为活化过硫酸氢钾（PMS）的催化剂，结果表明：当X-3B初始浓度为50 mg·L-1时，PMS=0.25 g·L-1、磁性OMS-2=0.25 g·L-1，4 h之内去除率可达93.66%。磁性OMS-2/PMS的浓度对SBR系统处理效果影响明显，低浓度磁性OMS-2/PMS（低于0.5 g·L-1）对SBR系统处理效果具有促进作用，高浓度OMS-2/PMS（大于或等于0.5 g·L-1）则会抑制SBR系统处理效果；此外，低浓度磁性OMS-2/PMS能提升SBR系统的缓冲能力。
    Abstract: For advanced treatment of dye wastewater, the sulfate radical based advanced oxidation process coupled with the sequencing batch reactor activated sludge process (SBR) was studied. The magnetic manganese oxide octahedral molecular sieve(OMS-2)was prepared as the catalyst for potassium peroxymonosulfate(PMS) activation. The results showed that, when the concentrations of X-3B, PMS and magnetic OMS-2 were 50 mg·L-1, 0.25 g·L-1 and 0.25 g·L-1, respectively, the removal of X-3B reached 93.66% within 4 h. The efficiency of SBR was strongly influenced by the magnetic OMS-2/PMS, which increased at low magnetic OMS-2/PMS concentrations (lower than 0.5 g·L-1), but decreased at high concentrations (equal or greater than 0.5 g·L-1). Besides, the buffer capacity of SBR could be promoted by low concentration of magnetic OMS-2/PMS.
  • [1] YAGUB M. T., SEN T. K., AFROZE S., et al. Dye and its removal from aqueous solution by adsorption: A review. Advances in Colloid and Interface Science, 2014, 209: 172-184
    [2] 贾佳祺, 李坤权, 陆凯, 等. 微波活化中孔酸性生物质炭对亚甲基蓝的吸附行为与机理. 环境工程学报, 2014, 8(3): 909-916 JIA Jiaqi, LI Kunquan, LU Kai, et al. Adsorption behavior and mechanism of methylene blue onto biomass-based mesoporous acid activated carbons by microwave heating. Chinese Journal of Environmental Engineering, 2014, 8(3): 909-916(in Chinese)
    [3] 林建伟, 王昕睿, 詹艳慧, 等. 阳离子表面活性剂改性四氧化三铁-沸石复合材料对水中刚果红的去除作用. 环境工程学报, 2014, 8(7): 2725-2732 LIN Jianwei, WANG Xinrui, ZHAN Yanhui, et al. Removal of Congo red from aqueous solution using cationic surfactant-modified magnetite/zeolite composite as adsorbent. Chinese Journal of Environmental Engineering, 2014, 8(7): 2725-2732(in Chinese)
    [4] 杨丽娟,魏杰,胡翔,等.Ce-PbO2/C电极的制备及其去除水中酸性红B.环境工程学报,2014, 8(3): 941-947 YANG Lijuan, WEI Jie, HU Xiang, et al. Preparation of Ce-PbO2/C and its application in removing Acid Red B from water. Chinese Journal of Environmental Engineering, 2014, 8(3): 941-947(in Chinese)
    [5] 杨林, 宋鑫, 王玉军, 等. 微电解预处理靛蓝牛仔布印染废水. 环境工程学报, 2013, 7(1): 268-272 YANG Lin, SONG Xin, WANG Yujun, et al. Pretreatment of indigo jean dyeing wastewater by iron-carbon micro-electrolysis process. Chinese Journal of Environmental Engineering, 2013, 7(1): 268-272(in Chinese)
    [6] 成岳, 焦创, 樊文井, 等. 包覆型纳米零价铁的制备及其去除水中的活性艳蓝. 环境工程学报, 2013, 7(1): 53-57 CHENG Yue, JIAO Chuang, FAN Wenjing, et al. Preparation of coated nanoscale zero-valent iron and its application in removing KN-R from wastewater. Chinese Journal of Environmental Engineering, 2013, 7(1): 53-57(in Chinese)
    [7] 黄萌萌, 买文宁, 李海松, 等. 铁炭微电解-Fe2+/K2S2O8降解甲基橙. 环境工程学报, 2014, 8(3): 935-940 HUANG Mengmeng, MAI Wenning, LI Haisong, et al. Degradation of methyl orange by iron carbon micro-electrolysis-Fe2+/K2S2O8. Chinese Journal of Environmental Engineering, 2014, 8(3): 935-940(in Chinese)
    [8] 薛懂, 李长波, 张洪林, 等. 絮凝-Fenton试剂氧化处理印染废水. 环境工程学报, 2014, 8(9): 3601-3606 XUE Dong, LI Changbo, ZHANG Honglin, et al. Oxidation treatment of printing and dyeing wastewater by flocculation-Fenton reagent. Chinese Journal of Environmental Engineering, 2014, 8(9): 3601-3606(in Chinese)
    [9] LUO Shilu, Duan Lian, SUN Binzhe, et al. Manganese oxide octahedral molecular sieve (OMS-2) as an effective catalyst for degradation of organic dyes in aqueous solutions in the presence of peroxymonosulfate. Applied Catalysis B: Environmental, 2015, 164: 92-99
    [10] PAN Fei, LUO Yin, ZHANG Lirong, et al. Degradation of Reactive Brilliant Red X-3B by zero-valent iron/activated carbon system in the presence of microwave irradiation. Water Science and Technology, 2011, 64(12): 2345-2351
    [11] 邓益强. 新型结构、形貌MFI型和OMS-2分子筛的可控合成、表征与催化应用. 长沙: 湖南大学博士学位论文, 2014 DENG Yiqiang. Controllabe synthesis, characterization and catalytic application of MFI and OMS-2 molecular sieves with novel structure and morphology. Changsha: Doctor Dissertation of Hunan University, 2014(in Chinese)
    [12] 王秀蘅, 任南琪, 王爱杰, 等. 铁锰离子对硝化反应的影响效应研究. 哈尔滨工业大学学报, 2003, 35(1): 122-125 WANG Xiuheng, REN Nanqi, WANG Aijie, et al. Effect of ferrous and manganese ion on nitrification. Journal of Harbin Institute of Technology, 2003, 35(1): 122-125(in Chinese)
    [13] DUAN Lian, SUN Binzhe, WEI Mingyu, et al. Catalytic degradation of Acid Orange 7 by manganese oxide octahedral molecular sieves with peroxymonosulfate under visible light irradiation. Journal of Hazardous Materials, 2015, 285: 356-365
    [14] 吴晓玉,储炬,李昌灵,等.Mn2+对菌株Y57生长及合成冠毒素的影响.江西农业大学学报,2007, 29(5): 827-829 WU Xiaoyu, CHU Ju, LI Changling, et al. Influence of Mn2+ on the cell growth and production of coronatine by strain Y57. Acta Agriculturae Universitatis Jiangxiensis, 2007, 29(5): 827-829(in Chinese)
    [15] 廖青, 李小明, 杨麒, 等. 好氧颗粒污泥的快速培养以及胞外多聚物对颗粒化的影响研究. 工业用水与废水, 2008, 39(4): 13-19 LIAO Qing, LI Xiaoming, YANG Qi, et al. Rapid cultivation of aerobic granular sludge and influence of extracellular polymeric substances on granulation. Industrial Water & Wastewater, 2008, 39(4): 13-19(in Chinese)
    [16] HUANG Lihui, YANG Tao, WANG Weiliang, et al. Effect of Mn2+ augmentation on reinforcing aerobic sludge granulation in a sequencing batch reactor. Applied Microbiology and Biotechnology, 2012, 93(6): 2615-2623

  • 期刊类型引用(2)

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    2. 王庆荣, 雷晓曼, 王赐眸, 尚禹佶, 吴媛媛, 夏东升, 潘飞. TNTs@CF吸附-紫外光催化降解亚甲基蓝. 武汉纺织大学学报. 2018(05): 26-32 . 百度学术

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出版历程
  • 收稿日期:  2015-05-10
  • 刊出日期:  2016-10-20
喻阳, 钟笑涵, 徐爱华, 夏东升, 曾庆福, 潘飞. 磁性OMS-2/SBR耦合处理活性染料X-3B废水[J]. 环境工程学报, 2016, 10(10): 5555-5560. doi: 10.12030/j.cjee.201504029
引用本文: 喻阳, 钟笑涵, 徐爱华, 夏东升, 曾庆福, 潘飞. 磁性OMS-2/SBR耦合处理活性染料X-3B废水[J]. 环境工程学报, 2016, 10(10): 5555-5560. doi: 10.12030/j.cjee.201504029
shu
YU Yang, ZHONG Xiaohan, XU Aihua, XIA Dongsheng, ZENG Qingfu, PAN Fei. Advanced treatment of simulated X-3B wastewater by coupling magnetic OMS-2 with SBR[J]. Chinese Journal of Environmental Engineering, 2016, 10(10): 5555-5560. doi: 10.12030/j.cjee.201504029
Citation: YU Yang, ZHONG Xiaohan, XU Aihua, XIA Dongsheng, ZENG Qingfu, PAN Fei. Advanced treatment of simulated X-3B wastewater by coupling magnetic OMS-2 with SBR[J]. Chinese Journal of Environmental Engineering, 2016, 10(10): 5555-5560. doi: 10.12030/j.cjee.201504029
shu

磁性OMS-2/SBR耦合处理活性染料X-3B废水

  • 1.  武汉纺织大学环境工程学院, 武汉 430073
  • 2.  武汉纺织大学生态苎麻产业关键技术湖北省协同创新中心, 武汉 430073
  • 收稿日期:  2015-05-10
基金项目:

国家科技支撑计划课题（2014BAC13B02）

湖北省教育厅中青年项目（Q20151603）

摘要: 为了深度处理印染废水，将基于硫酸根自由基的高级氧化法与序批式活性污泥法（SBR）相耦合；采用磁性氧化锰八面体分子筛（OMS-2）作为活化过硫酸氢钾（PMS）的催化剂，结果表明：当X-3B初始浓度为50 mg·L-1时，PMS=0.25 g·L-1、磁性OMS-2=0.25 g·L-1，4 h之内去除率可达93.66%。磁性OMS-2/PMS的浓度对SBR系统处理效果影响明显，低浓度磁性OMS-2/PMS（低于0.5 g·L-1）对SBR系统处理效果具有促进作用，高浓度OMS-2/PMS（大于或等于0.5 g·L-1）则会抑制SBR系统处理效果；此外，低浓度磁性OMS-2/PMS能提升SBR系统的缓冲能力。

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