2013 Volume 7 Issue 3
Article Contents
Abstract
References
Previous Article Next Article

Wu Dan, Zhu Lin, Wang Jian, Liu Qiang, Tang Yin, Gui Juduo. A biofilter treating hydrogen sulfide with high load and gas velocity in intermittent mode[J]. Chinese Journal of Environmental Engineering, 2013, 7(3): 1065-1071.
Citation: Wu Dan, Zhu Lin, Wang Jian, Liu Qiang, Tang Yin, Gui Juduo. A biofilter treating hydrogen sulfide with high load and gas velocity in intermittent mode[J]. Chinese Journal of Environmental Engineering, 2013, 7(3): 1065-1071.
shu

A biofilter treating hydrogen sulfide with high load and gas velocity in intermittent mode

  • 1.

    College of Environmental Science, Liaoning University, Shenyang 110036, China

  • 2.

    School of Municipal and Environmental Engineering, Harbin Institute of Technology, Harbin 150001, China

  • 3.

    Liaoning Academy of Environmental Sciences, Shenyang 110161, China

  • Received Date: 30/12/2011
    Accepted Date: 01/11/2011
    Available Online: 18/03/2013
    Fund Project:
  • Biological removal of hydrogen sulfide with high load and high gas velocity in intermittent mode in a biofilter, packed with the mixtures of chicken manure and polyethylene (PE) was investigated. With H2S inlet concentration of 3 000 mg/m3 and empty bed residence time (EBRT) of 20, 15, 10, 6.7 and 5 s, the average removal efficiencies were 100%, 100%, 96.5%, 89.2% and 90.5%, respectively. At the high gas velocity corresponding to EBRT of 5 s, the elimination capacity was 2 023 g/(m3·h) with high inlet load of 2 147 g/(m3·h), and H2S removal efficiencies could reach 94%. The removal kinetics was researched based on the Michaelis-Menten model. Two kinetic parameters were Ks with a value of 550 mg/m3, and Vm with a value of 6.8×104 g/(m3·d). The results showed that a good performance of the biofilter is obtained with high load and gas velocity under conditions of temperature from 17 to 24℃ and the moisture content ranges from 30% to 50%.
  • [1] Islam A. K. M. N., Hanaki K., Matsuo T. Fate of dissolved odorous compounds in sewage treatment plants.Wat. Sci. Tech., 1998, 38(3): 337-344

    Google Scholar Pub Med

    [2] Syed M., Soreanu G., Falletta P., et al.Removal of hydrogen sulfide from gas streams using biological processes-A review. Canadian Biosystems Engineering,2006, 48(5): 210-214

    Google Scholar Pub Med

    [3] 於建明, 沙昊雷, 陈建孟. 复合生物滤塔耦合处理含H2S和VOCs废气研究. 浙江工业大学学报,2008, 36 (3):254-259 Yu Jianming, Sha Wulei, Chen Jianmeng.Coupled biotreatment of waste gas containing H2S and VOCs by compound biofilter. Journal of Zhejinag University of Technology,2008, 36 (3): 254-259 (in Chinese)

    Google Scholar Pub Med

    [4] 梁永坤, 全燮, 陈景文, 等. 生物过滤法处理含氨废气研究. 环境科学学报, 2000, 20(5): 518-522 Liang Yongkun, Quan Xie, Chen Jingwen, et al.Biofiltration of ammonia-contaminated gas streams. Acta Scientiae Circumstantiae, 2000, 20(5): 518-522 (in Chinese)

    Google Scholar Pub Med

    [5] 李建军, 张甜甜, 孙国萍, 等. 生物过滤技术在恶臭污染治理中的应用研究. 环境工程学报,2008, 2(5): 712-715 Li Jianjun, Zhang Tiantian, Sun Guoping, et al.Study on application of biofilter in odor pollution control. Chinese Journal of Environmental Engineering,2008, 2(5): 712-715 (in Chinese)

    Google Scholar Pub Med

    [6] 王爱杰, 徐潇文, 任南琪, 等. 改进型生物脱臭滴滤塔对硫化氢和氨气的处理. 哈尔滨工业大学学报,2008, 40(2): 203-206 Wang Aijie, Xu Xiaowen, Ren Nanqi, et al.Efficiency of improved bio-trickling reactor for hydrogen sulfide and ammonia removal. Journal of Harbin Institute of Technology,2008, 40(2): 203-206 (in Chinese)

    Google Scholar Pub Med

    [7] 魏在山, 谢志荣. 生物法处理饲料恶臭废气工程应用研究. 环境工程,2010, 28(3): 85-87 Wei Zaishan, Xie Zhirong.Biological removal of industrial odor waste gas from aquatic feed production. Environmental Engineering,2010, 28(3): 85-87 (in Chinese)

    Google Scholar Pub Med

    [8] Rattanapan C., Kantachote D., Yan Y., et al. Hydrogen sulfide removal using granular activated carbon biofiltration inoculated with Alcaligenes faecalis T307 isolated from concentrated latex wastewater. International Biodeterioration and Biodegradation,2010, 64(5): 383-387

    Google Scholar Pub Med

    [9] 刘建伟, 黄力华, 马文林. 生物滴滤-生物过滤组合工艺处理汽车喷漆废气中试研究. 环境工程学报,2011, 5(4): 871-875 Liu Jianwei, Huang Lihua, Ma Wenlin.Pilot-study on treatment of paint spray booth emissions by integrating biotrickling filter with biofilter. Chinese Journal of Environmental Engineering,2011, 5(4): 871-875 (in Chinese)

    Google Scholar Pub Med

    [10] Lebrero R., Rodríguez E., García-Encina P. A., et al. A comparative assessment of biofiltration and activated sludge diffusion for odour abatement. Hazardous Materials,2011, 190(1-3): 622-630

    Google Scholar Pub Med

    [11] 张彭义, 余刚, 蒋展鹏, 等. 挥发性有机物和臭味的生物过滤处理. 环境污染治理技术与设备, 2000, 1(1): 1-7 Zhang Pengyi, Yu Gang, Dai Zhanpeng, et al.Treatment Of Volatile Organic Compounds And Odor By Biofitration. Techniques and Equipment for Environmental Pollution Control, 2000, 1(1): 1-7 (in Chinese)

    Google Scholar Pub Med

    [12] Omri I., Bouallagui H., Aouidi F., et al. H2S gas biological removal efficiency and bacterial community diversity in biofilter treating wastewater odor. Bioresource Technology,2011, 41(5): 512-524

    Google Scholar Pub Med

    [13] Kim J. H., Rene E. R., Park H. S. Biological oxidation of hydrogen sulfide under steady and transient state conditions in an immobilized cell biofilter. Bioresource Technology,2008, 99(3): 583-588

    Google Scholar Pub Med

    [14] Giri B. S., Mudliar S. N., Deshmukh S. C., et al. Treatment of waste gas containing low concentration of dimethyl sulphide (DMS) in a bench-scale biofilter. Bioresource Technology,2010, 101(7): 2185-2190

    Google Scholar Pub Med

    [15] 李莎璐, 蒋文举, 金燕, 等. 微生物脱臭研究应用进展. 环境科学与技术,2007, 30(5): 108-115 Li Shalu, Jiang Wenju, Jin Yan, et al.Advance on biotreatment of odors. Environmental Science & Technology,2007, 30(5): 108-115 (in Chinese)

    Google Scholar Pub Med

    [16] Chaiprapat S., Mardthing R., Kantachote D., et al. Removal of hydrogen sulfide by complete aerobic oxidation in acidic biofiltration. Process Biochemistry,2011, 46(1): 344-352

    Google Scholar Pub Med

    [17] Hassan A. A., Sorial G. A. Treatment of dynamic mixture of hexane and benzene vapors in a trickle bed air biofilter integrated with cyclic adsorption/desorption beds. Chemosphere,2011, 82(4): 521-528

    Google Scholar Pub Med

    [18] 张华新, 李顺义, 杨松波, 等. 多层生物滤塔净化硫化氢废气研究. 环境工程学报,2011, 5(1): 157-160 Zhang Huaxin, Li Shunyi, Yang Songbo, et al.Research on treatment of odor gas containing hydrogen sulfide by multilayer biofilter. Chinese Journal of Environmental Engineering,2011, 5(1): 157-160 (in Chinese)

    Google Scholar Pub Med

    [19] Duan H., Koe L. C. C., Yan R., et al. Biological treatment of H2S using pellet activated carbon as a carrier of microorganisms in a biofilter. Wa????げ???楡湲??栬椲渰攰猶攬??戰爨?嬴??崠′?栲甹渭朲?夳???????田慝渠枱“???倿???吠獈攜湋本????偿???旴瓤?懘汈?‖?椖漢璟爔斄愔瑶洮攠溯璃?潦昬′??猱甬戠?有??猩町戠?匷?愷渭搲?丹??獑畩扡????獮畧扳??据潧測琠慆楡湮楧渠杊?睮慹獩琬攠?杨慥獮攠獄?扮祧?捨潩?椠浥浴漠扡楬氮楒穥敭摯?捡敬氠汯獦?扨楹潤晲楯汧瑥敮爠???桦敩浤潥猠灢桹爠数???づ?ぴ???????????????? filter. Environmental Science,2011, 32(9): 2787-2793 (in Chinese)

    Google Scholar Pub Med

    [20] Fortuny M., Gamisans X., Deshusses M. A., et al. Operational aspects of the desulfurization process of energy gases mimics in biotrickling filters. Water Research,2011, 45(17): 5665-5674

    Google Scholar Pub Med

    [21] Jin Y. M., Veiga M. C., Kennes C.Effects of pH, CO2, and flow pattern on the autotrophic degradation of hydrogen sulfide in a biotrickling filter. Biotechnology and Bioengineering,2005, 92(4): 462-471

    Google Scholar Pub Med

    [22] Rattanapan C., Boonsawang P., Kantachote D. Removal of H2S in down-flow GAC biofiltration using sulfide oxidizing bacteria from concentrated latex wastewater. Bioresource Technology,2009, 100(1): 125-130

    Google Scholar Pub Med

    [23] 吴丹, 李法云, 陈晓阳, 等. 生物过滤法处理挥发性有机化合物研究进展. 科技导报,2009, 27(16): 99-103 Wu Dan, Li Fayun, Chen Xiaoyang, et al.Evaluation of Influencing Factors of Biofiltration of Volatile Organic Compounds. Science & Technology Review,2009, 27(16): 99-103 (in Chinese)

    Google Scholar Pub Med

    [24] Zhou Q., Yu L. H., Dyi-Hwa T., et al. A trickling fibrous-bed bioreactor for biofiltration of benzene in air. Chemical Technology and Biotechnology, 1998, 73(4): 359-368

    Google Scholar Pub Med

    [25] Erickson B. E. Environmentally friendly odor removal. Environmental Science and Technology, 2003, 37(13): 251

    Google Scholar Pub Med

    [26] 伍永钢, 赵敏. 生物滴滤床去除VOCs及恶臭物研究进展. 污染防治技术,2009, 22(5): 71-74 Wu Yonggang, Zhao Min.Study on VOCs and odors removal by biotrickling-bed reactor. Pollution Control Technology,2009, 22(5): 71-74 (in Chinese)

    Google Scholar Pub Med

    [27] Jin Y. M., Veiga M. C., Kennes C. Co-treatment of hydrogen sulfide and methanol in a single-stage biotrickling filter under acidic conditions. Chemosphere,2007, 68(6): 1186-1193

    Google Scholar Pub Med

    [28] 殷俊. 生物滤塔处理恶臭气体及微生物学机理. 杭州:浙江大学博士学位论文, 2004 Yin Jun. Biological Removal of Odorous Gases by Biofilter and Microbiological Mechanism. Hangzhou:Doctor Dissertation of Zhenjiang University

    Google Scholar Pub Med

  • 加载中
通讯作者: 陈斌, bchen63@163.com
  • 1. 

    沈阳化工大学材料科学与工程学院 沈阳 110142

  1. 本站搜索
  2. 百度学术搜索
  3. 万方数据库搜索
  4. CNKI搜索
Export Citation
PDF
XML

Article Metrics

Article views(2019) PDF downloads(1017) Cited by(0)

Access History

A biofilter treating hydrogen sulfide with high load and gas velocity in intermittent mode

  • Received Date: 30/12/2011
  • Accepted Date: 01/11/2011
  • Available Online: 18/03/2013
Fund Project:

Abstract: Biological removal of hydrogen sulfide with high load and high gas velocity in intermittent mode in a biofilter, packed with the mixtures of chicken manure and polyethylene (PE) was investigated. With H2S inlet concentration of 3 000 mg/m3 and empty bed residence time (EBRT) of 20, 15, 10, 6.7 and 5 s, the average removal efficiencies were 100%, 100%, 96.5%, 89.2% and 90.5%, respectively. At the high gas velocity corresponding to EBRT of 5 s, the elimination capacity was 2 023 g/(m3·h) with high inlet load of 2 147 g/(m3·h), and H2S removal efficiencies could reach 94%. The removal kinetics was researched based on the Michaelis-Menten model. Two kinetic parameters were Ks with a value of 550 mg/m3, and Vm with a value of 6.8×104 g/(m3·d). The results showed that a good performance of the biofilter is obtained with high load and gas velocity under conditions of temperature from 17 to 24℃ and the moisture content ranges from 30% to 50%.

    HTML

Reference (28)

Catalog

  • HTML

/

DownLoad:  Full-Size Img  PowerPoint
Return

All rights reserved: Reesearch Center for Eco-Environmental Sciences,Chinese Academy of Sciences Copyright © 1997-2016

Address:  Postcode: 100085 Phone: 010-62941074 E-mail: cjee@rcees.ac.cn

Supported by: Beijing Renhe Information Technology Co. Ltd  Technical support: info@rhhz.net