昆明市PM<sub>2.5</sub>中水溶性无机离子的化学特征及来源解析

朱若珲; 曹芳; 范美益

doi:10.7524/j.issn.0254-6108.2022120601

[1]

SUN Y L, WANG Z F, DU W, et al. Long-term real-time measurements of aerosol particle composition in Beijing, China: Seasonal variations, meteorological effects, and source analysis[J]. Atmospheric Chemistry and Physics, 2015, 15(17): 10149-10165. doi: 10.5194/acp-15-10149-2015

[2]

TIAN S L, PAN Y P, WANG Y S. Size-resolved source apportionment of particulate matter in urban Beijing during haze and non-haze episodes[J]. Atmospheric Chemistry and Physics, 2016, 16(1): 1-19. doi: 10.5194/acp-16-1-2016

[3]

TIAN M, WANG H B, CHEN Y, et al. Characteristics of aerosol pollution during heavy haze events in Suzhou, China[J]. Atmospheric Chemistry and Physics, 2016, 16(11): 7357-7371. doi: 10.5194/acp-16-7357-2016

[4]

徐沛华, 杨艳蓉, 刘梦迪, 等. 生物质燃烧排放颗粒物中水溶性有机物的光学特性[J]. 环境化学, 2022, 41(6): 2133-2142. doi: 10.7524/j.issn.0254-6108.2021022202 XU P H, YANG Y R, LIU M D, et al. Optical properties of water-soluble organic matters in particulate matter from biomass burning[J]. Environmental Chemistry, 2022, 41(6): 2133-2142 (in Chinese). doi: 10.7524/j.issn.0254-6108.2021022202

[5]

YU X N, MA J, AN J L, et al. Impacts of meteorological condition and aerosol chemical compositions on visibility impairment in Nanjing, China[J]. Journal of Cleaner Production, 2016, 131: 112-120. doi: 10.1016/j.jclepro.2016.05.067

[6]

CHEN P F, KANG S C, GUL C, et al. Seasonality of carbonaceous aerosol composition and light absorption properties in Karachi, Pakistan[J]. Journal of Environmental Sciences, 2020, 90: 286-296. doi: 10.1016/j.jes.2019.12.006

[7]

黄含含, 王羽琴, 李升苹, 等. 西安市PM_2.5中水溶性离子的季节变化特征[J]. 环境科学, 2020, 41(6): 2528-2535. HUANG H H, WANG Y Q, LI S P, et al. Seasonal variation of water-soluble ions in PM_2.5 in Xi’an[J]. Environmental Science, 2020, 41(6): 2528-2535 (in Chinese).

[8]

WANG H L, ZHU B, SHEN L J, et al. Water-soluble ions in atmospheric aerosols measured in five sites in the Yangtze River Delta, China: Size-fractionated, seasonal variations and sources[J]. Atmospheric Environment, 2015, 123: 370-379. doi: 10.1016/j.atmosenv.2015.05.070

[9]

尹璐, 董敏丽, 任芮芮, 等. 舟山市环境空气PM_2.5及水溶性离子污染特征分析[J]. 环境化学, 2019, 38(3): 556-564. doi: 10.7524/j.issn.0254-6108.2018050904 YIN L, DONG M L, REN R R, et al. Characteristics of PM_2.5 and water-soluble ions in ambient air in Zhoushan[J]. Environmental Chemistry, 2019, 38(3): 556-564 (in Chinese). doi: 10.7524/j.issn.0254-6108.2018050904

[10]

JACOBSON M C, HANSSON H C, NOONE K J, et al. Organic atmospheric aerosols: Review and state of the science[J]. Reviews of Geophysics, 2000, 38(2): 267-294. doi: 10.1029/1998RG000045

[11]

徐昶. 中国特大城市气溶胶的理化特性、来源及其形成机制[D]. 上海: 复旦大学, 2010: 53-63. XU C. Characteristics, source and the formation mechanism of aerosol in mega-city, China[D]. Shanghai: Fudan University, 2010: 53-63 (in Chinese).

[12]

WANG G H, ZHANG R Y, GOMEZ M E, et al. Persistent sulfate formation from London Fog to Chinese haze[J]. Proceedings of the National Academy of Sciences of the United States of America, 2016, 113(48): 13630-13635.

[13]

黄炯丽, 陈志明, 莫招育, 等. 基于高分辨率MARGA分析桂林市PM_2.5水溶性离子特征[J]. 中国环境科学, 2019, 39(4): 1390-1404. HUANG J L, CHEN Z M, MO Z Y, et al. Analysis of characteristics of water-soluble ions in PM_2.5 in Guilin based on the MARGA[J]. China Environmental Science, 2019, 39(4): 1390-1404 (in Chinese).

[14]

刘安康, 王红磊, 陈魁, 等. 南京市一次霾污染过程中水溶性离子分布特征[J]. 中国环境科学, 2019, 39(5): 1793-1803. LIU A K, WANG H L, CHEN K, et al. Distribution characteristics of water-soluble ions during a haze pollution process in Nanjing[J]. China Environmental Science, 2019, 39(5): 1793-1803 (in Chinese).

[15]

ALEXANDER B, SHERWEN T, HOLMES C D, et al. Global inorganic nitrate production mechanisms: Comparison of a global model with nitrate isotope observations[J]. Atmospheric Chemistry and Physics, 2020, 20(6): 3859-3877. doi: 10.5194/acp-20-3859-2020

[16]

WANG L T, HAO J M, HE K B, et al. A modeling study of coarse particulate matter pollution in Beijing: Regional source contributions and control implications for the 2008 summer olympics[J]. Journal of the Air & Waste Management Association, 2008, 58(8): 1057-1069.

[17]

ZHU J, XIA X, CHE H, et al. Study of aerosol optical properties at Kunming in southwest China and long-range transport of biomass burning aerosols from North Burma[J]. Atmospheric Research, 2016, 169: 237-247. doi: 10.1016/j.atmosres.2015.10.012

[18]

DENG X J, TIE X X, ZHOU X J, et al. Effects of Southeast Asia biomass burning on aerosols and ozone concentrations over the Pearl River Delta (PRD) region[J]. Atmospheric Environment, 2008, 42(36): 8493-8501. doi: 10.1016/j.atmosenv.2008.08.013

[19]

潘春梅. 中南半岛春季生物质燃烧对云南省空气质量影响研究[D]. 昆明: 云南师范大学, 2021: 32-51. PAN C M. Study on the impact of biomass burning on air quality in Yunnan Province in spring over indo-China peninsula[D]. Kunming: Yunnan Normal University, 2021: 32-51 (in Chinese).

[20]

周哆多. 云南地区上空UTLS区沙尘气溶胶传输过程及来源的数值模拟研究[D]. 昆明: 云南大学, 2019: 15-48. ZHOU D D. A simulation study on the source and transmission of the dust aerosol to the UTLS over the Yunnan Province[D]. Kunming: Yunnan University, 2019: 15-48 (in Chinese).

[21]

郭晓. 昆明市呈贡区及主城区干季大气PM_2.5的化学特征和来源对比[D]. 昆明: 云南师范大学, 2020: 17-29. GUO X. Comparison of chemical characteristics and sources of atmospheric PM_2.5 in Chenggong district and main urban district of Kunming in dry season[D]. Kunming: Yunnan Normal University, 2020: 17-29 (in Chinese).

[22]

ZHU Y H, HUANG L, LI J Y, et al. Sources of particulate matter in China: Insights from source apportionment studies published in 1987-2017[J]. Environment International, 2018, 115: 343-357. doi: 10.1016/j.envint.2018.03.037

[23]

古金霞, 吴丽萍, 霍光耀, 等. 天津市PM_2.5中水溶性无机离子污染特征及来源分析[J]. 中国环境监测, 2013, 29(3): 30-34. GU J X, WU L P, HUO G Y, et al. Pollution character and source of water-soluble inorganic ions in PM_2.5 over Tianjin[J]. Environmental Monitoring in China, 2013, 29(3): 30-34 (in Chinese).

[24]

贺瑶, 韩秀秀, 黄晓虎, 等. 南京市不同功能区冬季大气PM_2.5分布特征及其来源解析[J]. 环境科学学报, 2021, 41(3): 830-841. HE Y, HAN X X, HUANG X H, et al. Distribution characteristics and source apportionment of atmospheric PM_2.5 in winter season from different functional areas of Nanjing[J]. Acta Scientiae Circumstantiae, 2021, 41(3): 830-841 (in Chinese).

[25]

肖浩. 贵阳市PM_2.5水溶性无机离子组成特征及氮源解析[D]. 贵阳: 贵州大学, 2019: 23-51. XIAO H. Composition characteristics of water-soluble inorganic ions and nitrogen source analysis in PM_2.5 in Guiyang city[D]. Guiyang: Guizhou University, 2019: 23-51 (in Chinese).

[26]

高晓梅. 我国典型地区大气PM_2.5水溶性离子的理化特征及来源解析[D]. 济南: 山东大学, 2012: 48-97. GAO X M. Characterization and sources of PM_2.5 water-soluble ions in typical areas in China[D]. Jinan: Shandong University, 2012: 48-97 (in Chinese).

[27]

杨慧慧. 兰州市PM_2.5中水溶性离子的污染特征及来源解析[D]. 抚州: 东华理工大学, 2019: 15-41. YANG H H. Pollution characteristics and source analysis of water-soluble ions in PM_2.5 in Lanzhou city[D]. Fuzhou: East China Institute of Technology, 2019: 15-41 (in Chinese).

[28]

刘凡, 谭钦文, 江霞, 等. 成都市冬季相对湿度对颗粒物浓度和大气能见度的影响[J]. 环境科学, 2018, 39(4): 1466-1472. LIU F, TAN Q W, JIANG X, et al. Effect of relative humidity on particulate matter concentration and visibility during winter in Chengdu[J]. Environmental Science, 2018, 39(4): 1466-1472 (in Chinese).

[29]

ARIMOTO R, DUCE R A, SAVOIE D L, et al. Relationships among aerosol constituents from Asia and the north Pacific during PEM-west A[J]. Journal of Geophysical Research: Atmospheres, 1996, 101(D1): 2011-2023. doi: 10.1029/95JD01071

[30]

WANG Y, ZHUANG G S, TANG A H, et al. The ion chemistry and the source of PM_2.5 aerosol in Beijing[J]. Atmospheric Environment, 2005, 39(21): 3771-3784. doi: 10.1016/j.atmosenv.2005.03.013

[31]

吴丹, 蔺少龙, 杨焕强, 等. 杭州市PM_2.5中水溶性离子的污染特征及其消光贡献[J]. 环境科学, 2017, 38(7): 2656-2666. WU D, LIN S L, YANG H Q, et al. Pollution characteristics and light extinction contribution of water-soluble ions of PM_2.5 in Hangzhou[J]. Environmental Science, 2017, 38(7): 2656-2666 (in Chinese).

[32]

QIU X H, DUAN L, GAO J, et al. Chemical composition and source apportionment of PM₁₀ and PM_2.5 in different functional areas of Lanzhou, China[J]. Journal of Environmental Sciences, 2016, 40: 75-83. doi: 10.1016/j.jes.2015.10.021

[33]

SAFAI P D, BUDHAVANT K B, RAO P S P, et al. Source characterization for aerosol constituents and changing roles of calcium and ammonium aerosols in the neutralization of aerosol acidity at a semi-urban site in SW India[J]. Atmospheric Research, 2010, 98(1): 78-88. doi: 10.1016/j.atmosres.2010.05.011

[34]

XU L L, DUAN F K, HE K B, et al. Characteristics of the secondary water-soluble ions in a typical autumn haze in Beijing[J]. Environmental Pollution, 2017, 227: 296-305. doi: 10.1016/j.envpol.2017.04.076

[35]

张玉洽, 杨迎春, 李杰, 等. 东南亚生物质燃烧对我国春季PM_2.5质量浓度影响的数值模拟[J]. 环境科学研究, 2016, 29(7): 952-962. ZHANG Y Q, YANG Y C, LI J, et al. Modeling the impacts of biomass burning in Southeast Asia on PM_2.5 over China in spring[J]. Research of Environmental Sciences, 2016, 29(7): 952-962 (in Chinese).

[36]

CHEN C R, ZHANG H X, LI H Y, et al. Chemical characteristics and source apportionment of ambient PM_1.0 and PM_2.5 in a polluted city in North China plain[J]. Atmospheric Environment, 2020, 242: 117867. doi: 10.1016/j.atmosenv.2020.117867

[37]

黄敏. 上海浦东新区城区大气PM_2.5中水溶性离子污染特征研究[J]. 环境监控与预警, 2022, 14(2): 70-77. HUANG M. Study on pollution characteristics of water-soluble ions in PM_2.5 in Pudong new district[J]. Environmental Monitoring and Forewarning, 2022, 14(2): 70-77 (in Chinese).

[38]

DICKERSON R. Atmospheric chemistry and physics: From air pollution to climate change (second edition)[J]. Bulletin of the American Meteorological Society, 2009, 90(6): 868-870.

[39]

段卿. 南京北郊大气气溶胶化学组分特征分析[D]. 南京: 南京信息工程大学, 2015: 28-37. DUAN Q. The analysis of aerosol chemical composition characteristics in Nanjing northern suburb[D]. Nanjing: Nanjing University of Information Science & Technology, 2015: 28-37 (in Chinese).

[40]

DENG X L, SHI C E, WU B W, et al. Characteristics of the water-soluble components of aerosol particles in Hefei, China[J]. Journal of Environmental Sciences, 2016, 42: 32-40. doi: 10.1016/j.jes.2015.07.010

[41]

LI X R, WANG L L, JI D S, et al. Characterization of the size-segregated water-soluble inorganic ions in the Jing-Jin-Ji urban agglomeration: Spatial/temporal variability, size distribution and sources[J]. Atmospheric Environment, 2013, 77: 250-259. doi: 10.1016/j.atmosenv.2013.03.042

[42]

ZHAO J P, ZHANG F W, XU Y, et al. Characterization of water-soluble inorganic ions in size-segregated aerosols in coastal city, Xiamen[J]. Atmospheric Research, 2011, 99(3/4): 546-562.

[43]

XIE Z S, FAN C L, LU R, et al. Characteristics of ambient bioaerosols during haze episodes in China: A review[J]. Environmental Pollution, 2018, 243: 1930-1942. doi: 10.1016/j.envpol.2018.09.051

[44]

WANG J, ZHANG J S, LIU Z J, et al. Characterization of chemical compositions in size-segregated atmospheric particles during severe haze episodes in three mega-cities of China[J]. Atmospheric Research, 2017, 187: 138-146. doi: 10.1016/j.atmosres.2016.12.004

[45]

PERNIGOTTI D, BELIS C A, SPANÒ L. SPECIEUROPE: The European data base for PM source profiles[J]. Atmospheric Pollution Research, 2016, 7(2): 307-314. doi: 10.1016/j.apr.2015.10.007

[46]

昆明市统计局. 2021年昆明市国民经济和社会发展统计公报[EB/OL].