脉冲弧光放电等离子体水解活性污泥

曹颖, 姜楠, 段丽娟, 郭贺, 任景俞, 王璞, 周集体, 李杰, 吴彦. 脉冲弧光放电等离子体水解活性污泥[J]. 环境工程学报, 2018, 12(3): 956-965. doi: 10.12030/j.cjee.201709072
引用本文: 曹颖, 姜楠, 段丽娟, 郭贺, 任景俞, 王璞, 周集体, 李杰, 吴彦. 脉冲弧光放电等离子体水解活性污泥[J]. 环境工程学报, 2018, 12(3): 956-965. doi: 10.12030/j.cjee.201709072
CAO Ying, JIANG Nan, DUAN Lijuan, GUO He, REN Jingyu, WANG Pu, ZHOU Jiti, LI Jie, WU Yan. Activated sludge hydrolysis by pulse arc discharge plasma[J]. Chinese Journal of Environmental Engineering, 2018, 12(3): 956-965. doi: 10.12030/j.cjee.201709072
Citation: CAO Ying, JIANG Nan, DUAN Lijuan, GUO He, REN Jingyu, WANG Pu, ZHOU Jiti, LI Jie, WU Yan. Activated sludge hydrolysis by pulse arc discharge plasma[J]. Chinese Journal of Environmental Engineering, 2018, 12(3): 956-965. doi: 10.12030/j.cjee.201709072

脉冲弧光放电等离子体水解活性污泥

  • 基金项目:

    国家自然科学基金资助项目 (51477025)

Activated sludge hydrolysis by pulse arc discharge plasma

  • Fund Project:
  • 摘要: 活性污泥水解对提高污泥的稳定性、缩短厌氧消化时间和增大甲烷产率具有重要意义。研究了脉冲弧光放电等离子体(PADP)水解活性污泥方法,考察水解效果、影响因素和水解后的污泥性状。结果表明:随着峰值电压、频率和电导率的增加,污泥上清液营养物质含量呈增长趋势,溶胞率(R)升高;随着放电时间的增加,R增加,氨氮物质(NH4+-N)先增加后降低,可证明NH4+-N降解率逐渐上升且最终高于其释放率;污泥在14 kV、25 Hz、1 600 μS·cm-1条件下放电150 min,R增加到51.3%,NH4+-N、蛋白质和多糖等有机物大量释放;经过PADP处理,污泥沉降性降低,絮凝体结构改变,含固量和颗粒尺寸降低,污泥生物大量死亡,水解污泥生物由光滑、完整的表面结构变得粗糙、破裂,细胞壁(膜)受损明显,污泥发生水解。
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  • [1] MOWLA D, TRAN H N, ALLEN D G.A review of the properties of biosludge and its relevance to enhanced dewatering processes[J].Biomass & Bioenergy,2013,58(21):365-378 10.1016/j.biombioe.2013.09.002
    [2] XIANG Y, XIANG Y, WANG L.Cobalt-60 gamma-ray irradiation pretreatment and sludge protein for enhancing enzymatic saccharification of hybrid poplar sawdust[J].Bioresource Technology, 2016,221:9-14 10.1016/j.biortech.2016.09.032
    [3] RANI R U, KUMAR S, KALIAPPAN S, et al.Low temperature thermo-chemical pretreatment of dairy waste activated sludge for anaerobic digestion process[J].Bioresource Technology,2011,103(1): 415-424 10.1016/j.biortech.2011.09.124
    [4] BOUGRIER C, DELGENES J P,CARRERE H.Effects of thermal treatments on five different waste activated sludge samples solubilisation, physical properties and anaerobic digestion[J].Chemical Engineering Journal,2007,139(2):236-244 10.1016/j.cej.2007.07.099
    [5] NAH I W, KANG Y W, HWANG K Y, et al.Mechanical pretreatment of waste activated sludge for anaerobic digestion process[J].Water Research,2000,34(8):2362-2368 10.1016/S0043-1354(99)00361-9
    [6] APPELS L, HOUTMEYERS S, DEGREVE J, et al.Influence of microwave pre-treatment on sludge solubilization and pilot scale semi-continuous anaerobic digestion[J].Bioresource Technology,2012,128(1):598-603 10.1016/j.biortech.2012.11.007
    [7] DEVLIN D C, ESTEVES S R, DINSDALE R M, et al.The effect of acid pretreatment on the anaerobic digestion and dewatering of waste activated sludge[J].Bioresource Technology,2011,102(5):4076-4082 10.1016/j.biortech.2010.12.043
    [8] WAN J J, JING Y H, ZHANG S C, et al.Mesophilic and thermophilic alkaline fermentation of waste activated sludge for hydrogen production: Focusing on homoacetogenesis[J].Water Research,2016,102:524-532 10.1016/j.watres.2016.07.002
    [9] HASEGAWA S, SHIOTA N, KATSURA K, et al.Solubilization of organic sludge by thermophilic aerobic bacteria as a pretreatment for anaerobic digestion[J].Water Science & Technology,2000,41(3):163-169
    [10] SUN B M, YIN S E, GAO X D.Development prospects of non-thermal plasma technology used in the thermal power plants in China[C]//The American Society of Mechanical Engineers.International Conference on Energy Sustainability Collocated with the Heat Transfer and Interpack 2009 Conferences,2009:647-655
    [11] ZHANG H, ZHANG X D, WEI C C, et al.Microstructure characterization of microcrystalline silicon thin films deposited by very high frequency plasma-enhanced chemical vapor deposition by spectroscopic ellipsometry[J].Thin Solid Films,2011,520(2):861-865 10.1016/j.tsf.2011.04.166
    [12] WANG H J, GUO H, WU Q S, et al.Effect of activated carbon addition on H2O2 formation and dye decoloration in a pulsed discharge plasma system[J].Vacuum,2016,128:99-105 10.1016/j.vacuum.2016.03.015
    [13] GUO H, WANG H J, WU Q S, et al.Kinetic analysis of acid orange 7 degradation by pulsed discharge plasma combined with activated carbon and the synergistic mechanism exploration[J].Chemosphere,2016,159:221-227 10.1016/j.chemosphere.2016.05.092
    [14] CHOI H, JEONG S W, CHUNG Y J.Enhanced anaerobic gas production of waste activated sludge pretreated by pulse power technique[J].Bioresource Technology,2006,97(2):198-203 10.1016/j.biortech.2005.02.023
    [15] GAUNT L F, BEGGS C B, GEORGHIOU G E.Bactericidal action of the reactive species produced by gas-discharge nonthermal plasma at atmospheric pressure: A review[J].IEEE Transactions on Plasma Science,2006,34(4):1257-1269 10.1109/TPS.2006.878381
    [16] PIERCE B, MALOTT C, SAYLER G S, et al.Decontamination of media by a gaseous discharge at atmospheric pressure[C]//IEEE.IEEE Conference on Plasma Science,Anniverasy,1998
    [17] MORRISON G R.Microchemical determination of organic nitrogen with Nessler reagent[J].Analytical Biochemistry,1971,43(2):527-532 10.1016/0003-2697(71)90283-1
    [18] WEI Y J, LI K A, TONG S Y.A linear regression method for the study of the Coomassie brilliant blue protein assay[J].Talanta,1997,44(5):923-930 10.1016/S0039-9140(96)02140-6
    [19] FONG J, SCHAFFER F L, KIRK P L.The ultramicrodetermination of glycogen in liver:A comparison of the anthrone and reducing-sugar methods[J].Archives of Biochemistry & Biophysics,1953,45(2):319-326 10.1016/S0003-9861(53)80009-3
    [20] ASSOCIATION A P H.Standard methods for the examination of water and wastewater including bottom sediments and sludges[J].Journal of Clinical Laboratory Analysis,1967,53(3):361-386
    [21] DEVINS J C, RZAD S J, SCHWABE R J.Breakdown and prebreakdown phenomena in liquids[J].Journal of Applied Physics,1981,52(7):4531-4545 10.1063/1.329327
    [22] JONES H M, KUNHARDT E E.Development of pulsed dielectric breakdown in liquids[J].Journal of Physics D: Applied Physics,1995,28(1):178-188 10.1088/0022-3727/28/1/025
    [23] YU H, PERNI S, SHI J J, et al.Effects of cell surface loading and phase of growth in cold atmospheric gas plasma inactivation of Escherichia coli K12[J].Journal of Applied Microbiology,2006,101:1323-13300 10.1111/j.1365-2672.2006.03033.x
    [24] JIN Y, REN C S,XIU Z L,et al.Comparison of yeast inactivation treated in He, air and N2 DBD plasma[J].Plasma Science & Technology,2006,8(6):720-723 10.1088/1009-0630/8/6/21
    [25] VUKUSIC T, SHI M, HERCEG Z, et al.Liquid-phase electrical discharge plasmas with a silver electrode for inactivation of a pure culture of Escherichia coli in water[J].Innovative Food Science & Emerging Technologies,2016,38:407-413 10.1016/j.ifset.2016.07.007
    [26] LOCKE B R, SATO M, SUNKA P, et al.Electrohydraulic discharge and nonthermal plasma for water treatment[J].Industrial & Engineering Chemistry Research,2006,45(3):882-905 10.1021/ie050981u
    [27] SUAREZ-LGLESIAS O, URREA J L, OULEGO P, et al.Valuable compounds from sewage sludge by thermal hydrolysis and wet oxidation: A review[J].Science of the Total Environment,2017,584:921-934 10.1016/j.scitotenv.2017.01.140
    [28] ZHOU L F, HUANG B B, HUANG D W, et al.A feasible strategy for promoting activated sludge hydrolysis by using ironporphyrin modified Fe3O4 nanoparticles as an efficient biomimic catalyst[J].Chemical Engineering Journal,2015,280:248-255 10.1016/j.cej.2015.06.023
    [29] URREA J L, COLLADO S, LACA A, et al.Rheological behaviour of activated sludge treated by thermal hydrolysis[J].Journal of Water Process Engineering,2014,5:153-159 10.1016/j.jwpe.2014.06.009
    [30] XIN X D, HE J G, FENG J H, et al.Solubilization augmentation and bacterial community responses triggered by co-digestion of a hydrolytic enzymes blend for facilitating waste activated sludge hydrolysis process[J].Chemical Engineering Journal,2016,284:979-988 10.1016/j.cej.2015.09.060
    [31] LI D H, GANCZARCZYK J J.Structure of activated sludge flocs[J].Biotechnology & Bioengineering,1990,35(1):57-65
    [32] YANG S F, Li X Y.Influences of extracellular polymeric substances (EPS) on the characteristics of activated sludge under non-steady-state conditions[J].Process Biochemistry,2009,44(1):91-96 10.1016/j.procbio.2008.09.010
    [33] PAN X, LIU J, ZHANG D, et al.Binding of dicamba to soluble and bound extracellular polymeric substances (EPS) from aerobic activated sludge: A fluorescence quenching study[J].Journal of Colloid & Interface Science,2010,345(2):442-447 10.1016/j.jcis.2010.02.011
    [34] 王淑莹, 崔有为, 于德爽, 等. 无机盐对活性污泥沉降性的影响[J]. 环境工程, 2003, 21(5):7-9
    [35] PEYROUS R.The effect of relative humidity on ozone production by corona discharge in oxygen or air:A numerical simulation-Part I:oxygen[J].Ozone: Science & Engineering,1990,12(1):19-40 10.1080/01919519008552454
    [36] HOWARD D, STURTEVANT B.In vitro study of the mechanical effects of shock-wave lithotripsy[J].Ultrasound in Medicine & Biology,1997,23(7):1107-1122
    [37] WATTS R J, WASHINGTON D, HOWSAWKENG J, et al.Comparative toxicity of hydrogen peroxide, hydroxyl radicals, and superoxide anion to Escherichia coli[J].Advances in Environmental Research,2003,7(4):961-968 10.1016/S1093-0191(02)00100-4
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  • 刊出日期:  2018-03-22
曹颖, 姜楠, 段丽娟, 郭贺, 任景俞, 王璞, 周集体, 李杰, 吴彦. 脉冲弧光放电等离子体水解活性污泥[J]. 环境工程学报, 2018, 12(3): 956-965. doi: 10.12030/j.cjee.201709072
引用本文: 曹颖, 姜楠, 段丽娟, 郭贺, 任景俞, 王璞, 周集体, 李杰, 吴彦. 脉冲弧光放电等离子体水解活性污泥[J]. 环境工程学报, 2018, 12(3): 956-965. doi: 10.12030/j.cjee.201709072
CAO Ying, JIANG Nan, DUAN Lijuan, GUO He, REN Jingyu, WANG Pu, ZHOU Jiti, LI Jie, WU Yan. Activated sludge hydrolysis by pulse arc discharge plasma[J]. Chinese Journal of Environmental Engineering, 2018, 12(3): 956-965. doi: 10.12030/j.cjee.201709072
Citation: CAO Ying, JIANG Nan, DUAN Lijuan, GUO He, REN Jingyu, WANG Pu, ZHOU Jiti, LI Jie, WU Yan. Activated sludge hydrolysis by pulse arc discharge plasma[J]. Chinese Journal of Environmental Engineering, 2018, 12(3): 956-965. doi: 10.12030/j.cjee.201709072

脉冲弧光放电等离子体水解活性污泥

  • 1. 大连理工大学环境学院,大连 116024
  • 2. 大连理工大学电气工程学院,大连 116024
基金项目:

国家自然科学基金资助项目 (51477025)

摘要: 活性污泥水解对提高污泥的稳定性、缩短厌氧消化时间和增大甲烷产率具有重要意义。研究了脉冲弧光放电等离子体(PADP)水解活性污泥方法,考察水解效果、影响因素和水解后的污泥性状。结果表明:随着峰值电压、频率和电导率的增加,污泥上清液营养物质含量呈增长趋势,溶胞率(R)升高;随着放电时间的增加,R增加,氨氮物质(NH4+-N)先增加后降低,可证明NH4+-N降解率逐渐上升且最终高于其释放率;污泥在14 kV、25 Hz、1 600 μS·cm-1条件下放电150 min,R增加到51.3%,NH4+-N、蛋白质和多糖等有机物大量释放;经过PADP处理,污泥沉降性降低,絮凝体结构改变,含固量和颗粒尺寸降低,污泥生物大量死亡,水解污泥生物由光滑、完整的表面结构变得粗糙、破裂,细胞壁(膜)受损明显,污泥发生水解。

English Abstract

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