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聚丙烯中空纤维膜生物反应器净化复合芳香族VOCs

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王震文, 修光利, 詹天珍, 徐方圆, 吴来明, 张萍, 张大年. 聚丙烯中空纤维膜生物反应器净化复合芳香族VOCs[J]. 环境工程学报, 2013, 7(6): 2267-2272.
引用本文: 王震文, 修光利, 詹天珍, 徐方圆, 吴来明, 张萍, 张大年. 聚丙烯中空纤维膜生物反应器净化复合芳香族VOCs[J]. 环境工程学报, 2013, 7(6): 2267-2272.
shu
Wang Zhenwen, Xiu Guangli, Zhan Tianzhen, Xu Fangyuan, Wu Laiming, Zhang Ping, Zhang Danian. Treatment of mixtures of aromatic VOCs by a polypropylene hollow fiber menbrane bioreactor[J]. Chinese Journal of Environmental Engineering, 2013, 7(6): 2267-2272.
Citation: Wang Zhenwen, Xiu Guangli, Zhan Tianzhen, Xu Fangyuan, Wu Laiming, Zhang Ping, Zhang Danian. Treatment of mixtures of aromatic VOCs by a polypropylene hollow fiber menbrane bioreactor[J]. Chinese Journal of Environmental Engineering, 2013, 7(6): 2267-2272.
shu

聚丙烯中空纤维膜生物反应器净化复合芳香族VOCs

  • 1.

    华东理工大学, 国家环境保护化工过程环境风险评价与控制重点实验室, 上海 200237

  • 2.

    馆藏文物保护环境国家文物局重点科研基地(上海博物馆), 上海 200050

  • 基金项目:

    国家科技部"十一五"支撑计划资助(2010BAK67B15)

    中央高校基本科研业务费专项资金资助资助(WB1113005)

  • 中图分类号: X701

Treatment of mixtures of aromatic VOCs by a polypropylene hollow fiber menbrane bioreactor

  • 1.

    State Environmental Protection Key Laboratory of Risk Assessment and Control on Chemical Processes, East China University of Science & Technology, Shanghai 200237, China

  • 2.

    Key Scientific Research Base of Museum Environment, State Administration for Cultural Heritage, Shanghai Museum, Shanghai 200050, China

  • Fund Project:

摘要

  • 摘要: 采用中空纤维膜生物反应器(HFMBR)去除气态复合苯系物。挂膜后期,生物反应器的去除效率可以稳定达到80%左右(去除能力(EC)≥225 g/(m3·h))。研究了中空纤维膜生物反应器处理对于单一二甲苯以及混合二甲苯的性能,并且发现HFMBR对于去除单一二甲苯和混合二甲苯都有明显的效果,去除效率均达到90%以上;表明二甲苯之间竞争效应带来的相互抑制作用小。在低浓度的情况下,单一二甲苯和混合二甲苯的去除能力呈线性增加,在高浓度阶段,去除能力增加变缓。比较了混合二甲苯与甲苯联合降解,发现两者之间存在相互抑制作用,但相比传统生物反应器有明显的改善。与传统生物过滤系统比较而言,膜生物反应器有着很好的应用前景。
    Abstract: The hollow fiber membrane bioreactor (HFMBR) was used to remove gaseous mixtures of benzene series. During biofilm colonization, the removal efficiency and elimination capacity (EC) of bioreactor reached around 80%, 225 g/(m3·h), respectively. The performance of the HFMBR for treating single and mixed xylene were investigated, and it was found that the HFMBR can effectively treat both single and mixed xylenes, and the removal efficiency was over 90%, which indicated that the inhibition effect between xylene species was weak. The removal capacity of single and mixed xylenes increased linearly when the inlet concentration was lower while the increase became slower at higher concentration. Through comparing degradation of mixed xylene with toluene, the inhibition effect between them was found. However, the inhabitation was still lower than the conventional bioreactor. The membrane bioreactor therefore has a promising prospect for application compared with conventional biofiltration process.
  • [1] Mudliar S., Giri B., Padoley K., et al. Bioreactors for treatment of VOCs and odours:A review. Journal of Environmental Management, 2010,91(5):1039-1054
    [2] Khan F. I., Ghoshal A. K. Removal of volatile organic compounds from polluted air. Journal of Loss Prevention in the Process Industries, 2000,13(6):527-545
    [3] 都基峻, 季学李, 羌宁. 生物膜净化含苯废气的性能研究. 环境科学学报, 2005,25(3):401-404 Du Jijun, Ji Xueli, Qiang Ning.The performance of the biofilm to treat benzene in waste gas. Acta Scientiae Circumstantiae, 2005,25(3):401-404(in Chinese)
    [4] 孙珮石, 杨显万, 谢蕴国, 等. 生物法净化低浓度挥发性有机废气的动力学问题探讨. 环境科学学报, 1999,19(2):154-158 Sun Peishi,Yang Xianwan, Xie Yunguo, et al. Kinetics of purifying waste gases containing volatile organic compounds (VOC) in low concentration by using the biological methods. Acta Scientiae Circumstantiae, 1999,19(2):154-158(in Chinese)
    [5] 吕唤春, 潘洪明, 陈英旭. 低浓度挥发性有机废气的处理进展. 化工环保, 2001,21(6):324-327 Lu Huanchun, Pan Hongming, Chen Yingxu. Advanced in treatment of low concentration volatile organic compounds-Containing waste gas. Environmental Protection of Chemical Industry, 2001,21(6):324-327(in Chinese)
    [6] Reij M. W., Keurentjes J. T. F., Hartmans S. Membrane bioreaction for waste gas treatment. Journal of biotechnology, 1998,59(3):155-167
    [7] De Bo I. Membrane Biofiltartion of Single-Compound Waste Gas Streams. Belgium, Ghent: Universiteit Ghent, 2003
    [8] Luvsanjamba M., Kumar A., Van Langenhove H. Removal of dimethyl sulfide in a thermophilic membrane bioreactor. Journal of Chemical Technology and Biotechnology, 2008,83(9):1218-1225
    [9] Kumar A., Dewulf J., Langenhove H. V. Membrane-based biological waste gas treatment. Chemical Engineering Journal, 2008,136(2-3):82-91
    [10] 修光利, 张晓峰, 赵康, 等. 中空纤维膜生物反应器处理二甲苯废气. 环境工程学报, 2010,4(10):2287-2292 Xiu Guangli, Zhang Xiaofeng, Zhao Kang, et al. Treatment of waste gas containing xylene by a hollow fiber membrane bioreactor. Chinese Journal of Environmental Engineering, 2010,4(10):2287-2292(in Chinese)
    [11] 陈蓉, 曹明福, 王永忠, 等. 膜生物反应器处理甲苯废气的降解特性及传至过程强化. 环境工程学报, 2012,6(1):253-257 Chen Rong, Cai Mingfu, Wang Yongzhong, et al. Toluene biodegradation characteristics and mass transport enhancement in membrane bioreactors. Chinese Journal of Environmental Engineering, 2012,6(1):253-257(in Chinese)
    [12] Kennes C. K., Veiga M. C. Bioreactors for Waste Gas Treatment. London, Kluwer Academic Publishers, 2001
    [13] Shareefdeen Z, Singh A. Biotechnology for Odor and Air Pollution Control. Berlin: Springer, 2005
    [14] Devinny J. S., Deshusses M. A., Webster T. S. Biofiltration for Air Pollution Control. Boca Raton: Lewis Publishers, 1999
    [15] Kumar A., Yuan X., Ergas S., et al. Model of a polyethylene microporous hollow-fiber membrane biofilm reactor inoculated with Pseudomonas putida strain To1 1A for gaseous toluene removal. Bioresource Technology, 2010,101(7):2180-2184
    [16] Alvarez-Hornos F. J., Volckaert D., Heynderickx P. M., et al. Performance of a composite membrane bioreactor for the removal of ethyl acetate from waste air. Bioresource Technology, 2011,102(19):8893-8898
    [17] 徐利行. 中空纤维膜生物反应器净化挥发性有机气体的研究. 上海: 华东理工大学硕士学位论文, 2008 Xu Lihang. Studies on hollow fiber membrane bioreactor for biodegradation of VOCs. Shanghai: Master's Degree Thesis of East China Unversity of Science & Technology, 2008 (in Chinese)
    [18] Lu C. S., Chu W. C., Lin M. R. Removal of BTEX vaoor from waste gases by a trickle bed biofilter. Journal of the Air & Waste Management, 2000,50(3):411-417
    [19] 王娟, 钟秦, 郑曼曼, 等. 生物膜法净化甲苯二甲苯混合废气的研究. 环境科学与技术, 2006,29(6):91-93 Wang Juan, Zong Qin, Zheng Manman, et al. Purification of waste gas containing toluene and xylene using bio-film method. Environmental Science & Technology, 2006,29(6):91-93(in Chinese)
    [20] Zhao K., Xiu G. L., Xu L. H., et al. Biological treatment of mixtures of toluene and n-hexane vapours in a hollow fibre membrane bioreactor. Environmental Technology, 2011,32(6):617-623
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出版历程
  • 收稿日期:  2012-06-05
  • 刊出日期:  2013-06-11
王震文, 修光利, 詹天珍, 徐方圆, 吴来明, 张萍, 张大年. 聚丙烯中空纤维膜生物反应器净化复合芳香族VOCs[J]. 环境工程学报, 2013, 7(6): 2267-2272.
引用本文: 王震文, 修光利, 詹天珍, 徐方圆, 吴来明, 张萍, 张大年. 聚丙烯中空纤维膜生物反应器净化复合芳香族VOCs[J]. 环境工程学报, 2013, 7(6): 2267-2272.
shu
Wang Zhenwen, Xiu Guangli, Zhan Tianzhen, Xu Fangyuan, Wu Laiming, Zhang Ping, Zhang Danian. Treatment of mixtures of aromatic VOCs by a polypropylene hollow fiber menbrane bioreactor[J]. Chinese Journal of Environmental Engineering, 2013, 7(6): 2267-2272.
Citation: Wang Zhenwen, Xiu Guangli, Zhan Tianzhen, Xu Fangyuan, Wu Laiming, Zhang Ping, Zhang Danian. Treatment of mixtures of aromatic VOCs by a polypropylene hollow fiber menbrane bioreactor[J]. Chinese Journal of Environmental Engineering, 2013, 7(6): 2267-2272.
shu

聚丙烯中空纤维膜生物反应器净化复合芳香族VOCs

  • 1. 华东理工大学, 国家环境保护化工过程环境风险评价与控制重点实验室, 上海 200237
  • 2. 馆藏文物保护环境国家文物局重点科研基地(上海博物馆), 上海 200050
  • 收稿日期:  2012-06-05
基金项目:

国家科技部"十一五"支撑计划资助(2010BAK67B15)

中央高校基本科研业务费专项资金资助资助(WB1113005)

摘要: 采用中空纤维膜生物反应器(HFMBR)去除气态复合苯系物。挂膜后期,生物反应器的去除效率可以稳定达到80%左右(去除能力(EC)≥225 g/(m3·h))。研究了中空纤维膜生物反应器处理对于单一二甲苯以及混合二甲苯的性能,并且发现HFMBR对于去除单一二甲苯和混合二甲苯都有明显的效果,去除效率均达到90%以上;表明二甲苯之间竞争效应带来的相互抑制作用小。在低浓度的情况下,单一二甲苯和混合二甲苯的去除能力呈线性增加,在高浓度阶段,去除能力增加变缓。比较了混合二甲苯与甲苯联合降解,发现两者之间存在相互抑制作用,但相比传统生物反应器有明显的改善。与传统生物过滤系统比较而言,膜生物反应器有着很好的应用前景。

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