不同粒径泥沙理化特性对磷吸附过程的影响

崔双超, 丁爱中, 潘成忠, 李长嘉, 鄢正红, 刘奕慧, 郝丽芬. 不同粒径泥沙理化特性对磷吸附过程的影响[J]. 环境工程学报, 2013, 7(3): 863-868.
引用本文: 崔双超, 丁爱中, 潘成忠, 李长嘉, 鄢正红, 刘奕慧, 郝丽芬. 不同粒径泥沙理化特性对磷吸附过程的影响[J]. 环境工程学报, 2013, 7(3): 863-868.
Cui Shuangchao, Ding Aizhong, Pan Chengzhong, Li Changjia, Yan Zhenghong, Liu Yihui, Hao Lifen. Effect of sediment physicochemical properties on phosphorus sorption for different size particles[J]. Chinese Journal of Environmental Engineering, 2013, 7(3): 863-868.
Citation: Cui Shuangchao, Ding Aizhong, Pan Chengzhong, Li Changjia, Yan Zhenghong, Liu Yihui, Hao Lifen. Effect of sediment physicochemical properties on phosphorus sorption for different size particles[J]. Chinese Journal of Environmental Engineering, 2013, 7(3): 863-868.

不同粒径泥沙理化特性对磷吸附过程的影响

  • 基金项目:

    国家自然科学基金资助项目(41040028)

    中央高校基本科研业务费专项

    国家"水体污染控制与治理"科技重大专项(2009ZX07212-002)

    北京市委、市政府重点工作及区县政府应急预启动项目(Z10110605540000)

  • 中图分类号: X703

Effect of sediment physicochemical properties on phosphorus sorption for different size particles

  • Fund Project:
  • 摘要: 以北京大兴南海子湖表层沉积物为研究对象,测试分析了0.147~0.246 mm(细砂)、0.074~0.147 mm(极细砂)、0.0385~0.0740 mm(粉粒)和R2>0.90)。粒径对单位质量泥沙吸附磷量具有明显影响,粉粒粘粒混合物>粉粒>细砂>极细砂。总体上,泥沙有机质(OM)、TP、Fe、Al、Ca和Mn含量随粒径的减小而增大,且粘粒对其影响较大。不同粒径泥沙(OM)、Fe、Al、Ca和Mn含量之间存在极显著正相关关系(PXm)和饱和吸附量(Cse)具有正效应,其中Al含量对该参数的影响更为显著。这说明泥沙对磷的吸附行为可能受到粒径和化学成分的共同影响。
  • [1] Withers P. J. A., Jarvie H. P. Delivery and cycling of phosphorus in rivers: A review. Sci. Total. Environ.,2008,400(1-3): 379-395
    [2] 张宪伟,潘纲,王晓丽,等. 内蒙古段黄河沉积物对磷的吸附特征研究. 环境科学,2009,30(1):172-177 Zhang. X. W., Pan. G., Wang X. L., et al. Characteristics of phosphorus sorption on yellow river sediments from Inner Mongolia reach. Environmental Science,2009,30(1):172-177 (in Chinese)
    [3] Pan G., Michael D. K., Barak H. Adsorption-desorption of phosphate on airborne dust and riverborne particulates in east Mediterranean Seawater. Eviron.Sci.Technol,2002,36(16):3519-3524
    [4] Ozacar M. Equilibrium and kinetic modeling of adsorption of phosphorus on calcined alunite. Adsorption,2003,9(2):125-132
    [5] Chien S. H., Clayton W. R. Application of elovich equation to the kinetics of phosphate release and sorption in soils. Soil Science Society of America Journal,1980,44(2):265-268
    [6] 吕平毓,黄文典,李嘉. 河流悬移质对含磷污染物吸附试验研究. 水利水电技术,2005,36(10):93-96 Lü P. Y., Huang W. D., Li J. Study on adsorption experiment for phosphorous pollutant with suspended sediment. Water Resources and Hydropower Technology,2005,36(10):93-96(in Chinese)
    [7] 袁东海,张孟群,高士祥,等. 几种粘土矿物和粘粒土壤吸附净化磷素的性能和机理. 环境化学,2005,24(1):7-11 Yuan D. H., Zhang M. Q., Gao S.X. The abilities and mechanisms of adsorption phosphorus in some clay minerls and soils. Environmental Chemistry,2005,24(1):7-11(in Chinese)
    [8] 金相灿,屠清瑛. 湖泊富营养化调查规范(第2版). 北京:中国环境科学出版社,1990
    [9] 周孝德,韩世平,陈惠君. 环境因素对滇池底泥磷吸附的影响. 水利学报,1998,(增刊):12-17 Zhou X. D., Han S. P., Chen H. J. The influences of environmental factors on phosphate sorption by sediments in lake Dianchi. Journal of Hydraulic Engineering,1998,(supplement): 12-17(in Chinese)
    [10] 王圣瑞,金相灿,赵海超,等. 湖泊沉积物物中水溶性有机质对吸附磷的影响. 土壤学报,2005,42(5):806-808 Wang S. R., Jin X. C., Zhao H. C. Effect of DOM on phosphate sorption in lake sediments. Acta Pedologica Sinica,2005,42(5):806-808(in Chinese)
    [11] Stone M., Mudroch A. Effect of Particle-size, chemistry and mineralogy of river sediments on Phosphate adsorption. Environmental Technology Letters,1989,10(5):501-510
    [12] Stone P. M., Walling D. E. The particle-size selectivity of sediment mobilization from Devon Hillslopes. Advances in Hillslope Processes,1996,1(2):507-527
    [13] 王圣瑞,赵海超,周小宁,等. 五里湖与贡湖不同粒径沉积物中有机质、总氮和磷形态分布研究. 环境科学研究,2004, 17(增刊):11-14 Wang S. R., Zhao H. C., Zhou X. N., et al. Study on the organic matter,totai nitrogen and phosphorus form distribution of different particle size fractions in the sediments from Wuli Lake and Gonghu Lake. Research of Environmental Sciences,2004,17(supplement):11-14(in Chinese)
    [14] 金相灿,王圣瑞,赵海超,等. 五里湖和贡湖不同粒径沉积物吸附磷实验研究. 环境科学研究,2004,17(增刊):6-9 Jin X. C., Wang S. R., Zhao H. C., et al. Study on the phosphate sorption of the different particle size fractions in the sediments from Wuli Lake and Gonghu Lake. Research of Environmental Sciences,2004,17(supplement):6-9(in Chinese)
    [15] 戴纪翠,宋金明,李学刚等. 胶州湾不同形态磷的沉积记录及生物可利用性研究. 环境科学,2007,28(5):930-936 Dai J. C., Song J. M.,Li X. G., et al. Sediment record of phosphorus and the primary study of its bioavailability in Jiaozhou Bay sediment. Environmental Science,2007,28(5):930-936(in Chinese)
    [16] Lijklema L. Interaction of ortho-phosphate with iron(III) and aluminum hydroxides. Environ. Sci. Technol.,1980,14(5):537-541
    [17] Zhang J. Z., Huang X. L. Relative importance of solid-phase phosphorus and iron on the sorption behavior of sediments. Environ. Sci. Technol.,2007,41(8):2789-2795
    [18] 王晓丽,潘纲,包华影,等. 黄河中下游沉积物对磷酸盐的吸附特征. 环境科学,2008,29(8):2137-2142 Wang X. L., Pan G., Bao H. Y., et al. Phosphate sorption characteristics onto sediments in the middle and lower reaches of the Yellow River. Environmental Science,2008,29(8):2137-2142(in Chinese)
    [19] Katarina B., Erasmus O., Elisabetta B. Phosphorus sorption in relation to soil properties in some cultivated Swedish soil. Nutrient Cycling in Agroecosystems,2001,59(1):39-46
    [20] Subramanlam V., Singh B. R. Phosphorus supplying capacity of heavily fertilized soils. 1. Phosphorus adsorption characteristics and phosphorus fractionation. Nutr Cycl Agroecosys,1997,47(2):115-122
    [21] 刘光菘. 土壤理化性质与剖面描述. 北京:中国标准出版社,1996
    [22] 国家环境保护总局.水和废水监测分析方法(第4版). 北京:中国环境科学出版社,2002
    [23] 鲍士旦. 土壤农化分析. 南京:农业出版社,1986
    [24] Chen S.H., Clayton W. R. Application of Elovich equation to the kinetics of phosphorus release and sorption in soils. Soil Science of America Journal,1980,44(1): 265-268
    [25] Pavlatou A., Polyzopoulos N. A. The role of diffusion in the kinetics of phosphate desorption:The relevance of the Elovich equation. European Journal of Soil Science,1988,39(3):425-436
    [26] Bergamasehi B.A., Tsamakis E., Ceil R.G., et al. The effect of grain size and surface area on organic matter, lignin and carbohydrate concentration, and molecular composition in Peru Margin sediments. Geochimica et Cosmochimica Acta,1997,61(6):1247-1260
    [27] 朱广伟,秦伯强,高光,等. 长江中下游浅水湖泊沉积物中磷的形态及其与水相磷的关系. 环境科学学报,2004,24(3):381-388 Zhu G. W., Qin B. Q., Gao G., et al. Fractionation of phosphorus in sediments and its relation with soluble phosphorus contents in shallow lakes located in the middle and lower reaches of Changjiang River. Acta Scientiae Circumstantiae,2004,24(3):381-388(in Chinese)
  • 加载中
计量
  • 文章访问数:  2526
  • HTML全文浏览数:  1437
  • PDF下载数:  1342
  • 施引文献:  0
出版历程
  • 收稿日期:  2012-02-11
  • 刊出日期:  2013-03-18
崔双超, 丁爱中, 潘成忠, 李长嘉, 鄢正红, 刘奕慧, 郝丽芬. 不同粒径泥沙理化特性对磷吸附过程的影响[J]. 环境工程学报, 2013, 7(3): 863-868.
引用本文: 崔双超, 丁爱中, 潘成忠, 李长嘉, 鄢正红, 刘奕慧, 郝丽芬. 不同粒径泥沙理化特性对磷吸附过程的影响[J]. 环境工程学报, 2013, 7(3): 863-868.
Cui Shuangchao, Ding Aizhong, Pan Chengzhong, Li Changjia, Yan Zhenghong, Liu Yihui, Hao Lifen. Effect of sediment physicochemical properties on phosphorus sorption for different size particles[J]. Chinese Journal of Environmental Engineering, 2013, 7(3): 863-868.
Citation: Cui Shuangchao, Ding Aizhong, Pan Chengzhong, Li Changjia, Yan Zhenghong, Liu Yihui, Hao Lifen. Effect of sediment physicochemical properties on phosphorus sorption for different size particles[J]. Chinese Journal of Environmental Engineering, 2013, 7(3): 863-868.

不同粒径泥沙理化特性对磷吸附过程的影响

  • 1. 北京师范大学水科学研究院,教育部地下水污染控制与修复工程研究中心,污染场地风险模拟与 修复北京市重点实验室, 北京 100875
  • 2. 太原电力高等专科学校, 太原 030013
基金项目:

国家自然科学基金资助项目(41040028)

中央高校基本科研业务费专项

国家"水体污染控制与治理"科技重大专项(2009ZX07212-002)

北京市委、市政府重点工作及区县政府应急预启动项目(Z10110605540000)

摘要: 以北京大兴南海子湖表层沉积物为研究对象,测试分析了0.147~0.246 mm(细砂)、0.074~0.147 mm(极细砂)、0.0385~0.0740 mm(粉粒)和R2>0.90)。粒径对单位质量泥沙吸附磷量具有明显影响,粉粒粘粒混合物>粉粒>细砂>极细砂。总体上,泥沙有机质(OM)、TP、Fe、Al、Ca和Mn含量随粒径的减小而增大,且粘粒对其影响较大。不同粒径泥沙(OM)、Fe、Al、Ca和Mn含量之间存在极显著正相关关系(PXm)和饱和吸附量(Cse)具有正效应,其中Al含量对该参数的影响更为显著。这说明泥沙对磷的吸附行为可能受到粒径和化学成分的共同影响。

English Abstract

参考文献 (27)

返回顶部

目录

/

返回文章
返回